作者机构:
[Huang, Tao; Zhou, Lulu; Yang, Chun-Hai] Changshu Inst Technol, Sch Mat Engn, Changshu 215500, Peoples R China.;[Huang, Tao] Changshu Inst Technol, Suzhou Key Lab Funct Ceram Mat, Changshu 215500, Peoples R China.;[Huang, Tao] China Univ Min & Technol, Sch Chem Engn & Technol, Xuzhou 221116, Jiangsu, Peoples R China.;[Zhang, Shu-wen] Univ South China, Nucl Resources Engn Coll, Hengyang 421001, Peoples R China.
通讯机构:
[Tao Huang] S;School of Materials Engineering, Changshu Institute of Technology, 215500, China<&wdkj&>Suzhou Key Laboratory of Functional Ceramic Materials, Changshu Institute of Technology, Changshu, 215500, China<&wdkj&>School of Chemical Engineering & Technology, China University of Mining and Technology, Xuzhou, Jiangsu, 221116, China
期刊:
Separation and Purification Technology,2023年307:122873 ISSN:1383-5866
通讯作者:
Dai, Zhongran(dzr1122@126.com)
作者机构:
[Ding, Dexin; Li, Le; Dai, Zhongran; Chen, Lijie; Lian, Junjie] Univ South China, Key Discipline Lab Natl Def Biotechnol Uranium Min, Hengyang 421001, Peoples R China.;[Gao, Yuan] China Univ Min & Technol, Sch Chem Engn & Technol, Xuzhou 221116, Jiangsu, Peoples R China.
通讯机构:
[Zhongran Dai] K;Key Discipline Laboratory for National Defense for Biotechnology in Uranium Mining and Hydrometallurgy, University of South China, Hengyang 421001, China
期刊:
Journal of Physics: Conference Series,2023年2587(1):012031 ISSN:1742-6588
作者机构:
[Fan Wu] College of Civil Engineering, University of South China, Hunan, Hengyang, China;Key Discipline Lab. for National Defence of Biotechnology in Uranium Mining and Hydrometallurgy, University of South China, Hengyang;421001, China;[Shuibo Xie] College of Civil Engineering, University of South China, Hunan, Hengyang, China <&wdkj&> Key Discipline Lab. for National Defence of Biotechnology in Uranium Mining and Hydrometallurgy, University of South China, Hengyang;[Shuibo Xie] 421001, China
摘要:
<jats:title>Abstract</jats:title>
<jats:p>In this study, a green and efficient persimmon tannin functionalized polyacrylonitrile fiber (PAN-TETA-PT) was prepared and used to treat U(VI). The influence of pH value, adsorption temperature and time, and fiber material dosage on the adsorption U(VI) of PAN-TETA-PT fibers were investigated, and the kinetics, isotherm, and thermodynamics of fibers were analyzed. When the pH is 6, the temperature is 30°C, and the fiber dosage is 0.2 g·L<jats:sup>−1</jats:sup>, the adsorption rate of PAN-TETA-PT fibers to U(VI) was 96.5%, and the U(VI) adsorption capacity was 159.75 mg/g. The kinetic and isothermal studies show that the adsorption of PAN-TETA-PT fibers to U(VI) is chemisorbed and multilayer adsorption. The thermodynamic analysis reflects that the PAN-TETA-PT is spontaneously endothermic for the adsorbed U(VI).</jats:p>
期刊:
Environmental Science: Water Research & Technology,2023年9(5):1480-1490 ISSN:2053-1400
通讯作者:
Ding, Dexin(dingdxzzz@163.com)
作者机构:
[Ding, Dexin; Zhang, Hui; Hu, Nan; Ding, Yang; Liu, Yalan] Univ South China, Key Discipline Lab Natl Def Biotechnol Uranium Min, Hengyang 421001, Peoples R China.;[Ding, Dexin; Zhang, Hui; Hu, Nan; Ding, Yang; Liu, Yalan] Hunan Prov Key Lab Green Dev Technol Extremely Low, Hengyang 421001, Peoples R China.
通讯机构:
[Dexin Ding] K;Key Discipline Laboratory for National Defense for Biotechnology in Uranium Mining and Hydrometallurgy, University of South China, Hengyang 421001, China<&wdkj&>Hunan Province Key Laboratory of Green Development Technology for Extremely Low Grade Uranium Resources, Hengyang 421001, China
期刊:
Journal of Physics: Conference Series,2023年2587(1):012047 ISSN:1742-6588
作者机构:
College of Civil Engineering, University of South China, Hengyang, Hunan, China;Key Discipline Lab. for National Defence of Biotechnology in Uranium Mining and Hydrometallurgy, University of South China, Hengyang;421001, China;[Haibo Zhang; Shuibo Xie] College of Civil Engineering, University of South China, Hengyang, Hunan, China <&wdkj&> Key Discipline Lab. for National Defence of Biotechnology in Uranium Mining and Hydrometallurgy, University of South China, Hengyang;[Haibo Zhang; Shuibo Xie] 421001, China
摘要:
<jats:title>Abstract</jats:title>
<jats:p>Persimmon tannin modified chitosan (PT-CS) microspheres were synthesized by a water bath method using sodium tripolyphosphate (STPP) as a cross-linking agent for the removal of U(VI) from wastewater. The results showed that the optimal preparation conditions for PT-CS were a ratio of PT to CS mass of 4:1 and a reaction temperature of 80°C. When the initial concentration of U(VI) was 5 mg/L, and the pH value was 1.5, the PT-CS was injected at 0.06 g/L, and the reaction was 2.5 h. The removal rate of U(VI) from water reached 99.2%. The results of the deep removal test of U(VI) from rare earth wastewater showed that the concentrations of U(VI) in the combined wastewater and extraction wastewater were reduced from 4.42 mg/L and 2.12 mg/L to within 0.02 mg/L at pH 2.0, respectively. In contrast, the removal rate of high concentrations of Ca<jats:sup>2+ i</jats:sup>n the wastewater reached 99%, meeting the emission standards of the rare earth industry.</jats:p>
期刊:
Colloids and Surfaces A: Physicochemical and Engineering Aspects,2022年642:128606 ISSN:0927-7757
通讯作者:
Xie, Shuibo(xiesbmr@263.net)
作者机构:
[Guo, Yu; Xie, Shuibo; Wang, Chenxu; Wang, Lingzhi; Liu, Haiyan] Univ South China, Coll Civil Engn, Hengyang 421001, Peoples R China.;[Xie, Shuibo] Univ South China, Key Discipline Lab Natl Def Biotechnol Uranium Mi, Hengyang 421001, Peoples R China.;[Liu, Xiaoyang] Water Resources Bur Ziyang Dist, Yiyang City 413001, Peoples R China.
通讯机构:
[Shuibo Xie] C;College of Civil Engineering, University of South China, Hengyang 421001, China<&wdkj&>Key Discipline Laboratory for National Defence of Biotechnology in Uranium Mining and Hydrometallurgy, University of South China, Hengyang 421001, China
作者机构:
[Ding, Dexin; He, Liu; Deng, Qinwen; Wang, Yongdong] Univ South China, Key Discipline Lab Natl Def Biotechnol Uranium Mi, Hengyang 421001, Peoples R China.;[He, Liu; Deng, Qinwen; Wang, Fan] Univ South China, Hengyang Key Lab Soil Pollut Control & Remediat, Hengyang, Peoples R China.;[Ding, Dexin; He, Liu; Deng, Qinwen; Wang, Fan; Wang, Yongdong] Univ South China, Sch Resources Environm & Safety Engn, Hengyang, Peoples R China.
通讯机构:
[Qinwen Deng] K;Key Discipline Laboratory for National Defense for Biotechnology in Uranium Mining and Hydrometallurgy, University of South China, Hengyang, P.R. China. Hengyang Key Laboratory of Soil Pollution Control and Remediation, University of South China, Hengyang, P.R. China. School of Resources, Environment and Safety Engineering, University of South China, Hengyang, P.R. China.
关键词:
Macleaya cordata (Willd.) R. Br.;phytoremediation;uranium tailings
作者机构:
[Liu, Yuelin] Univ South China, Key Discipline Lab Natl Def Biotechnol Uranium Mi, Hengyang 421001, Peoples R China.;[Liu, Yuelin] Hunan Univ Technol, Sch Civil Engn, Zhuzhou 412007, Peoples R China.;[Wu, Shanshan; Xie, Shuibo; Liu, Yingjiu] Univ South China, Hunan Prov Key Lab Pollut Control & Resources Reu, Hengyang 421001, Peoples R China.;[Liu, Jun] Hunan Univ Technol, Sch Life Sci & Chem, Hunan Key Lab Biomed Nanomat & Devices, Zhuzhou 412007, Peoples R China.;[Xie, Shuibo] Univ South China, Sch Civil Engn, Hengyang 421001, Peoples R China.
通讯机构:
[Xie, Shuibo] U;Univ South China, Hunan Prov Key Lab Pollut Control & Resources Reu, Hengyang 421001, Peoples R China.;Univ South China, Sch Civil Engn, Hengyang 421001, Peoples R China.
摘要:
Photocatalytic technology is a valid solution for the remediation of wastewater containing uranium. In this study, the synthesis of Z-scheme g-C(3)N(4)/TiO(2) catalysts was made by a thermal synthetic approach for photocatalytic U(vi) reduction. The characterization results revealed the successful synthesis of g-C(3)N(4)/TiO(2) nanostructures. The g-C(3)N(4) surface was uniformly coated with TiO(2) nanoparticles. The depletion of U(vi) in water evaluated the photocatalytic activity of g-C(3)N(4)/TiO(2) under UV light irradiation. The photocatalytic tests showed that g-C(3)N(4)/TiO(2) exhibited more effective photocatalytic activity than the raw materials (1.64 and 56.97 times higher than TiO(2)(P25) and g-C(3)N(4), respectively). Besides, a pseudo-first-order model was followed by the experimental kinetic data for the photocatalytic process. Moreover, g-C(3)N(4)/TiO(2) still presented high photocatalytic activity after four reacting cycles. Based on these experiment results, the improved photocatalytic activity could be attributed to the Z-scheme mechanism, which decreased the recombination of photo-produced electrons and holes. The synthesis of these g-C(3)N(4)/TiO(2) nanomaterials provides a facile and inexpensive method for treating wastewater containing U(vi).
通讯机构:
[Dexin Ding] K;Key Discipline Laboratory for National Defense for Biotechnology in Uranium Mining and Hydrometallurgy, University of South China, Hengyang 421001, China
作者机构:
[Huang, Tao; Liu, Long-fei; Zhou, Lulu] Changshu Inst Technol, Sch Mat Engn, Changshu 215500, Jiangsu, Peoples R China.;[Huang, Tao] Changshu Inst Technol, Suzhou Key Lab Funct Ceram Mat, Changshu 215500, Jiangsu, Peoples R China.;[Huang, Tao] China Univ Min & Technol, Sch Chem Engn & Technol, Xuzhou 221116, Jiangsu, Peoples R China.;[Zhang, Shu-wen] Univ South China, Nucl Resources Engn Coll, Hengyang 421001, Peoples R China.
通讯机构:
[Huang, Tao] C;Changshu Inst Technol, Sch Mat Engn, Changshu 215500, Jiangsu, Peoples R China.
关键词:
Green rust;Functionalized composite cementitious material;Geopolymer;Chromate;Granulated blast furnace slag;Fly ash
摘要:
Green rust functionalized geopolymer of composite cementitious materials (GR-CCM) was synthesized to improve the adsorption and subsequent stabilization/solidification of chromate in a holistic operating system. The initial pH in solution exhibited the most significant effect on the chromate removal by GR-CCM among three adsorption factors. The maximum monolayer adsorption capacity and theoretical saturation capacity of GR-CCM for Cr(VI) in the acidic condition were 55.01 mg/g and 41.70 mg/g, respectively. Amorphousness brought by loading GR weakened the crystallinity of composite cementitious materials (CCM), which enhanced the adsorption capacity of CCM and boosted the solidification process. The mixed-valent iron species in the GR-CCM not only directly engaged in the adsorption and reduction of chromate also positively strengthened the solidification of Cr species during the whole treatment. This study facilitates the application of GRs on the geopolymer materials and demonstrates the combination of adsorption and immobilization for the treatment of other potential heavy metal contamination. (C) 2020 Elsevier Ltd. All rights reserved.
作者机构:
[胡南; 陈雪; 张辉; 李艾书; 李广悦; 王永东; 丁德馨] Key Discipline Laboratory for National Defense for Biotechnology in Uranium Mining and Hydrometallurgy, University of South China, Hengyang;421001, China;[胡南; 陈雪; 张辉; 李艾书; 李广悦; 王永东; 丁德馨] 421001, China
作者机构:
[伍随意; 胡俊毅; 贺俊钦; 王国华; 荣丽杉; 金远远] Hunan Provincial Key Laboratory of Pollution Control and Resources Technology, University of South China, Hengyang;421001, China;[李仕友] Key Discipline Laboratory for National Defence for Biotechnology in Uranium Mining and Hydrometallurgy, University of South China, Hengyang;[伍随意; 李仕友; 胡俊毅; 贺俊钦; 王国华; 荣丽杉; 金远远] 421001, China
通讯机构:
[Li, S.] K;Key Discipline Laboratory for National Defence for Biotechnology in Uranium Mining and Hydrometallurgy, China
作者机构:
[刘玉龙; 扶海鹰; 胡南; 李广悦; 喻清; 丁德馨] Key Discipline Laboratory for National Defense for Biotechnology in Uranium Mining and Hydrometallurgy, University of South China, Hengyang;421001, China;China General Nuclear Power Group(CGN) Uranium Resources Co. Ltd., Beijing;100029, China;[刘玉龙] 421001, China <&wdkj&> China General Nuclear Power Group(CGN) Uranium Resources Co. Ltd., Beijing