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EtOH-catalyzed electrosynthesis of imidazolidine-fused sulfamidates from N-sulfonyl ketimines, N-arylglycines and formaldehyde

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成果类型:
期刊论文
作者:
Lu, Yu-Han;Mu, Si-Yu;Li, Hong-Xia;Jiang, Jun;Wu, Chao;...
通讯作者:
He, WM
作者机构:
[Li, Hong-Xia; Lu, Yu-Han; Mu, Si-Yu] Univ South China, Hengyang Med Sch, Hengyang 421001, Peoples R China.
[Wu, Chao; Zhou, Min-Hang; Lu, Yu-Han; He, Wei-Min; Ouyang, Wen-Tao; Jiang, Jun; He, WM] Univ South China, Sch Chem & Chem Engn, Hengyang 421001, Peoples R China.
通讯机构:
[He, WM ] U
Univ South China, Sch Chem & Chem Engn, Hengyang 421001, Peoples R China.
语种:
英文
期刊:
Green Chemistry
ISSN:
1463-9262
年:
2023
卷:
25
期:
14
页码:
5539-5542
基金类别:
We are grateful for the financial support from the University of South China.
机构署名:
本校为第一且通讯机构
院系归属:
化学化工学院
摘要:
With formaldehyde as an atom-economical carbonyl synthon, the EtOH-catalyzed electrochemical multicomponent synthesis of various imidazolidine-fused sulfamidates was developed. A wide range of products were obtained in good to excellent yields under organic oxidant-free, energy-saving and mild conditions. The mechanistic study revealed that the in situ generated ethoxide played a crucial role in pro...

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