Customizing the Crystal Facet of Carbon-Encapsulated Nickel Catalyst for Selective and Durable Electrocatalytic CO2 Reduction to CO

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成果类型：

期刊论文

作者：

Chen, Fei;Deng, Liu;He, Haichuan;Wang, Liqiang;Yang, Minghui;...

通讯作者：

Liu, YN;He, HC

作者机构：

[Yang, Minghui; Chen, Fei; Liu, You-Nian; Deng, Liu] Cent South Univ, Coll Chem & Chem Engn, Hunan Prov Key Lab Micro & Nano Mat Interface Sci, Changsha 410083, Hunan, Peoples R China.

[Chen, Fei] Xinjiang Med Univ, Coll Pharm, Xinjiang Key Lab Nat Med Act Components & Drug Rel, Urumqi 830017, Xinjiang, Peoples R China.

[Wang, Liqiang] Zhengzhou Univ, Henan Prov Ind Technol Res Inst Resources & Mat, Sch Mat Sci & Engn, Zhengzhou 450001, Henan, Peoples R China.

[He, Haichuan] Univ South China, Sch Chem & Chem Engn, Hengyang 421001, Hunan, Peoples R China.

[Liu, You-Nian] Hangzhou Normal Univ, Coll Mat Chem & Chem Engn, Hangzhou 311121, Zhejiang, Peoples R China.

通讯机构：

[He, HC ] U

[Liu, YN ] C

Cent South Univ, Coll Chem & Chem Engn, Hunan Prov Key Lab Micro & Nano Mat Interface Sci, Changsha 410083, Hunan, Peoples R China.

Univ South China, Sch Chem & Chem Engn, Hengyang 421001, Hunan, Peoples R China.

Hangzhou Normal Univ, Coll Mat Chem & Chem Engn, Hangzhou 311121, Zhejiang, Peoples R China.

语种：

英文

期刊：

Industrial & Engineering Chemistry Research

ISSN：

0888-5885

年：

2025

DOI：

10.1021/acs.iecr.4c05006

基金类别：

National Natural Science Foundation of China [22238013, 22178393]; National Natural Science Foundation of China [320808]; Postdoctoral Science Foundation of Central South University [2023JJ40706]; Natural Science Foundation of Hunan Province; High-Performance Computing Center of Central South University

机构署名：

本校为通讯机构

院系归属：

化学化工学院

摘要：

Carbon-supported non-noble metal-based catalysts display remarkable catalytic activity and cost-effectiveness in electrochemical CO2 reduction reaction (eCO2RR). However, precise control of the crystal facet of metal catalysts and prevention of deactivation caused by agglomeration remain challenges. Herein, a novel dual-function customized strategy is presented for the preparation of the N-doped carbon-supported Ni-based porous catalyst with carbon-encapsulated Ni(111) nanoparticles (Ni(111)@C-NDPC), through carbonizing the self-assembly of protein-Ni-ions networks and ethylenediaminetetraacet...

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Customizing the Crystal Facet of Carbon-Encapsulated Nickel Catalyst for Selective and Durable Electrocatalytic CO2 Reduction to CO

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