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K doped defective g-C3N4 decorated with cyano group for boosting visible-light driven photocatalytic removal of uranium

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成果类型:
期刊论文
作者:
Dai, Zhongran*;Chen, Lijie;Zhang, Weilin;Liang, Beichao;Gao, Yuan;...
通讯作者:
Dai, Zhongran;Li, L;Gao, Y
作者机构:
[Dai, Zhongran; Liang, Beichao; Li, Le; Chen, Lijie] Univ South China, Key Discipline Lab Natl Def Biotechnol Uranium Min, Hengyang 421001, Peoples R China.
[Gao, Yuan; Gao, Y] China Univ Min & Technol, Sch Chem Engn & Technol, Xuzhou 221116, Jiangsu, Peoples R China.
[Li, Le; Zhang, Weilin] Univ South China, Coll Publ Hlth, Hengyang Med Sch, Hengyang 421001, Hunan, Peoples R China.
通讯机构:
[Dai, ZR; Li, L ] U
[Gao, Y ] C
Univ South China, Key Discipline Lab Natl Def Biotechnol Uranium Min, Hengyang 421001, Peoples R China.
China Univ Min & Technol, Sch Chem Engn & Technol, Xuzhou 221116, Jiangsu, Peoples R China.
语种:
英文
关键词:
U(VI);Removal;Adsorption;Photoreduction;Wastewater
期刊:
Separation and Purification Technology
ISSN:
1383-5866
年:
2024
卷:
338
页码:
126537
基金类别:
CRediT authorship contribution statement Zhongran Dai: Writing – original draft, Resources, acquisition. Lijie Chen: Investigation, Conceptualization. Weilin Zhang: Validation, Investigation. Beichao Liang: Validation, Resources. Yuan Gao: Writing – review & editing, Methodology. Le Li: Writing – review & editing, Supervision, acquisition.
机构署名:
本校为第一且通讯机构
院系归属:
核资源工程学院
公共卫生学院
摘要:
Utilizing elemental doping and defect engineering are effective means to enhance the efficiency of g-C3N4 materials for photocatalytic removal of uranium. In this investigation, we synthesized a defective g-C3N4 photocatalyst co-decorated with K+ doping and cyano groups (KHCN) through a straightforward one-step alkali etching process. The alkali etching not only enhances the specific surface area to improve the adsorption of uranium by KHCN but also significantly accelerates the photocatalytic removal of uranium through the introduction of K+ and cyano groups. The KHCN can almost completely re...

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