Optimization of crystallization dynamics in wide-bandgap bromine-iodine perovskite films for high-performance perovskite-organic tandem solar cells

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成果类型：

期刊论文

作者：

Song, Zonglong;Wang, Jiangfeng;Bao, Yuqi;Zeng, Jie;Wang, Deng;...

通讯作者：

Wang, Xingzhu;Xu, BM;Wang, XZ;Liu, YS

作者机构：

[Xu, Baomin; He, Siru; Wang, Xingzhu; Jiang, Bo; Liu, Zhixin; He, Jiang; Wang, Deng; Wang, XZ; Wang, Jiangfeng; Bao, Yuqi; Zhu, Peide; Song, Zonglong; Zeng, Jie] Southern Univ Sci & Technol, Dept Mat Sci & Engn, Shenzhen 518055, Peoples R China.

[Xu, Baomin; Wang, Xingzhu; Wang, XZ] Southern Univ Sci & Technol, Shenzhen Engn Res & Dev Ctr Flexible Solar Cells, Dept Mat Sci & Engn, Shenzhen 518055, Peoples R China.

[Xu, Baomin; Wang, Xingzhu; Wang, XZ] Southern Univ Sci & Technol, SUSTech Energy Inst Carbon Neutral, Shenzhen 518055, Peoples R China.

[Wang, Xingzhu; Wang, XZ] Shenzhen Putai Technol Co Ltd, Shenzhen 518110, Peoples R China.

[Wang, Xingzhu; Wang, XZ] Univ South China, Sch Elect Engn, Hengyang 421001, Peoples R China.

通讯机构：

[Liu, YS ] N

[Xu, BM ; Wang, XZ ; Wang, XZ] S

Southern Univ Sci & Technol, Dept Mat Sci & Engn, Shenzhen 518055, Peoples R China.

Southern Univ Sci & Technol, Shenzhen Engn Res & Dev Ctr Flexible Solar Cells, Dept Mat Sci & Engn, Shenzhen 518055, Peoples R China.

Southern Univ Sci & Technol, SUSTech Energy Inst Carbon Neutral, Shenzhen 518055, Peoples R China.

语种：

英文

期刊：

Energy & Environmental Science

ISSN：

1754-5692

年：

2025

DOI：

10.1039/D5EE00264H

基金类别：

Science, Technology and Innovation Commission of Shenzhen Municipality [SGDX20230116091649013, JCYJ20220818100211025, KCXST20221021111616039]; Shenzhen Science and Technology Innovation Committee [2023B1515120031, 2022A1515110413]; Guangdong Basic and Applied Basic Research Foundation [2023JJ50132]; Natural Science Foundation of Hunan Province, China [61904076, 62204108, 62104158]; National Natural Science Foundation of China [GDRC202113]; Natural Science Foundation of Top Talent of SZTU [202403AP140015]; Project for Building a Science and Technology Innovation Center Facing South Asia [G03034K001]; SUSTech Energy Institute for Carbon Neutrality (High level of special funds); SUSTech Core Research Facilities; Center for Computational Science and Engineering at SUSTech

机构署名：

本校为通讯机构

院系归属：

电气工程学院

摘要：

The development of efficient and stable wide-bandgap (WBG) bromine–iodine halide perovskites (Br > 20%) is crucial for enhancing the performance of tandem solar cells. Nonetheless, phase separation of I–Br in WBG perovskites under illumination and heating significantly hinders the advancement of tandem devices. This phenomenon is primarily attributed to the uneven spatial distribution of halide ions in WBG films. Moroxydine hydrochloride was introduced into 1.85 eV I–Br mixed WBG perovskite films, effectively optimizing the crystallization d...

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Optimization of crystallization dynamics in wide-bandgap bromine-iodine perovskite films for high-performance perovskite-organic tandem solar cells

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