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Efficient visible-light-driven photoreduction of U(VI) by carbon dots modified porous g-C3N4

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成果类型:
期刊论文
作者:
Dai, Zhongran;Zhao, Shang;Lian, Junjie;Li, Le;Ding, Dexin
通讯作者:
Dexin Ding
作者机构:
[Ding, Dexin; Li, Le; Dai, Zhongran; Zhao, Shang; Lian, Junjie] Univ South China, Key Discipline Lab Natl Def Biotechnol Uranium Min, Hengyang 421001, Peoples R China.
通讯机构:
[Dexin Ding] K
Key Discipline Laboratory for National Defense for Biotechnology in Uranium Mining and Hydrometallurgy, University of South China, Hengyang 421001, China
语种:
英文
关键词:
Adsorption;Photoreduction;Removal;U(VI);Wastewater
期刊:
Separation and Purification Technology
ISSN:
1383-5866
年:
2022
卷:
298
页码:
121590
基金类别:
The morphology of g-C3N4 and CNCD-2 were characterized by TEM. As shown in Fig. 1a, the g-C3N4 has a typical layered porous structure. The microstructure of g-C3N4 was well maintained after CDs modification (Fig. 1b), and some CDs nanoparticles with a diameter of about 1 nm were observed on the surface of CNCD-2 (Fig. 1c) [42]. Next, the TEM elemental mapping of CNCD-2-U (CNCD-2 after photoreduction of uranium) was shown in Fig. 1e-1i. The main elemental constituent of CNCD-2-U was C, N, O and
机构署名:
本校为第一机构
院系归属:
核资源工程学院
摘要:
The efficient removal of uranium from radioactive wastewater is of great significance for the ecological environment safety and sustainable development of nuclear energy. Herein, the carbon dots modified porous graphitic carbon nitride (CNCD) was fabricated and used for photoreduction of U(VI) under visible LED light irradiation. The removal rate of U(VI) by CNCD-2 could reach more than 95 % over a wide range of U(VI) concentration. In addition, the CNCD-2 showed excellent selectivity and recyclability for photoreduction of U (VI). Further mechanism studies showed that the high photocatalysis ...

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