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A hydrolytically stable europium-organic framework for the selective detection of radioactive Th4+ in aqueous solution

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成果类型:
期刊论文
作者:
Song, Liping;Liu, Wei;Wang, Yanlong;Chen, Lanhua;Wang, Xiao-Feng*;...
通讯作者:
Wang, Xiao-Feng;Wang, Shuao
作者机构:
[Song, Liping; Wang, Xiao-Feng] Univ South China, Sch Chem & Chem Engn, Hengyang 421001, Peoples R China.
[Song, Liping; Wang, Xiao-Feng] Univ South China, Hunan Prov Engn Res Ctr Radioact Control Technol, Hengyang 421001, Peoples R China.
[Chen, Lanhua; Liu, Wei; Song, Liping; Wang, Yanlong; Wang, Shuao] Soochow Univ, State Key Lab Radiat Med & Protect, Sch Radiol & Interdisciplinary Sci RAD X, Collaborat Innovat Ctr Radiat Med Jiangsu Higher, Suzhou 215123, Peoples R China.
[Chen, Lanhua; Liu, Wei; Song, Liping; Wang, Yanlong; Wang, Shuao] Soochow Univ, Sch Radiat Med & Protect, Suzhou 215123, Peoples R China.
通讯机构:
[Wang, Xiao-Feng] U
[Wang, Shuao] S
Univ South China, Sch Chem & Chem Engn, Hengyang 421001, Peoples R China.
Univ South China, Hunan Prov Engn Res Ctr Radioact Control Technol, Hengyang 421001, Peoples R China.
Soochow Univ, State Key Lab Radiat Med & Protect, Sch Radiol & Interdisciplinary Sci RAD X, Collaborat Innovat Ctr Radiat Med Jiangsu Higher, Suzhou 215123, Peoples R China.
语种:
英文
期刊:
CrystEngComm
ISSN:
1466-8033
年:
2019
卷:
21
期:
22
页码:
3471-3477
基金类别:
This work was supported by grants from the National Science Foundation of China (21825601, 21790370, 21790374, and 11375082), the Science Challenge Project (TZ2016004), the Postgraduate research innovation fund program of Hunan Province (2018KYY045), the Postgraduate Research & Practice Innovation Program of Jiangsu Province (KYCX17_2018), and the Hunan Province Engineering Research Center of Radioactive Control Technology in Uranium Mining and Metallurgy & Hunan Province Engineering Technology Research Center of Uranium Tailings Treatment Technology-University of South China (2019YKZX1004).
机构署名:
本校为第一且通讯机构
院系归属:
化学化工学院
摘要:
Thorium is not only a promising candidate for developing next generation nuclear fuel but also a potential radioactive contaminant. Efficient detection of thorium contamination is critically important in both nuclear science and environmental protection. We present here a 3D luminescent europium organic framework [Eu2(FDC)3(DMA)2]·4H2O (compound 1), which exhibits excellent hydrolytic stability and features highly selective detection capacity (KSV = 6.68 × 104) towards radioactive Th4+ ions among the selected monovalent, divalent and tervalen...

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