Enhanced activation of peroxymonosulfate by nickel sulfide with sulfur vacancies for ultrafast organic pollutants degradation: Roles of active sites and mechanism

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成果类型：

期刊论文

作者：

Luo, Cai-Wu*;Jiang, Liang;Li, Xian-Feng;Wan, Qiang-Mao;Jiang, Tian-Jiao;...

通讯作者：

Luo, Cai-Wu;Xie, C

作者机构：

[Xie, C; Luo, Cai-Wu; Xie, Chao; Zhao, Run-Ze; Jiang, Liang; Li, Xian-Feng; Guo, Jing-Qian; Mao, Sen-Ping; Luo, CW] Univ South China, Sch Resources Environm & Safety Engn, Hengyang 421000, Peoples R China.

[Wan, Qiang-Mao] China Natl Nucl Corp, Nucl Ind Coll, Beijing 102413, Peoples R China.

[Xie, Chao; Jiang, Tian-Jiao] Univ South China, Sch Nucl Sci & Technol, Hengyang 421000, Peoples R China.

通讯机构：

[Xie, C ; Luo, CW] U

Univ South China, Sch Resources Environm & Safety Engn, Hengyang 421000, Peoples R China.

语种：

英文

关键词：

Nickel sulfide;Organic pollutants;Peroxymonosulfate;Sulfur;Vacancies

期刊：

Environmental Pollution

ISSN：

0269-7491

年：

2025

卷：

372

页码：

125789

DOI：

10.1016/j.envpol.2025.125789

基金类别：

CRediT authorship contribution statement Cai-Wu Luo: Writing – review & editing, Resources, Project administration, acquisition, Data curation, Conceptualization. Liang Jiang: Writing – original draft, Formal analysis, Data curation. Xian-Feng Li: Data curation. Qiang-Mao Wan: Software. Tian-Jiao Jiang: Methodology. Sen-Ping Mao: Validation. Jing-Qian Guo: Methodology. Run-Ze Zhao: Validation. Chao Xie: Resources.

机构署名：

本校为第一且通讯机构

院系归属：

核科学技术学院

摘要：

The transition metal sulfide-activated peroxymonosulfate (PMS) has been proven to be a promising alternative for removing organic pollutants in wastewater. However, the interaction among active sites was not fully elucidated. To clarify this issue, a simple nickel sulfide with sulfur vacancies (NSHC10-400) via the hydrothermal-calcination successive treatments was successfully fabricated and employed for activating PMS for Acid Orange II (AOII) removal. The results showed that the Ni 2+ , reductive sulfur species and sulfur vacancies acted as main active sites on the activation of PMS. Due to ...

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Enhanced activation of peroxymonosulfate by nickel sulfide with sulfur vacancies for ultrafast organic pollutants degradation: Roles of active sites and mechanism

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