A ternary mechanism for the facilitated transfer of metal ions onto metal-organic frameworks: implications for the \'\'versatility\'\' of these materials as solid sorbents - 成果

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A ternary mechanism for the facilitated transfer of metal ions onto metal-organic frameworks: implications for the ''versatility'' of these materials as solid sorbents

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成果类型：

期刊论文

作者：

Bu, Xiyuan;Tian, Ming;Wang, Hongqing;Wang, Lin;Yuan, Liyong;...

通讯作者：

Liyong Yuan

作者机构：

[Yuan, Liyong; Shi, Weiqun; Bu, Xiyuan; Wang, Lin; Tian, Ming] Chinese Acad Sci, Inst High Energy Phys, Lab Nucl Energy Chem, Beijing 100049, Peoples R China.

[Wang, Hongqing; Tian, Ming] Univ South China, Sch Chem & Chem Engn, Hengyang 421001, Peoples R China.

通讯机构：

[Liyong Yuan] L

Laboratory of Nuclear Energy Chemistry, Institute of High Energy Physics, Chinese Academy of Sciences, Beijing, China

语种：

英文

关键词：

U(VI);metal-organic frameworks;adsorption mechanism;metal node

期刊：

化学科学与工程前沿：英文版

ISSN：

2095-0179

年：

2022

卷：

期：

页码：

1632-1642

DOI：

10.1007/s11705-022-2187-6

基金类别：

This work was supported by the National Natural Science Foundation of China (Grant Nos. U20B2019, 21790373 and 21790370) and the National Science Fund for Distinguished Young Scholars (Grant No. 21925603).

机构署名：

本校为其他机构

院系归属：

化学化工学院

摘要：

Although metal—organic frameworks offer a new platform for developing versatile sorption materials, yet coordinating the functionality, structure and component of these materials remains a great challenge. It depends on a comprehensive knowledge of a “real sorption mechanism”. Herein, a ternary mechanism for U(VI) uptake in metal—organic frameworks was reported. Analogous MIL-100s (Al, Fe, Cr) were prepared and studied for their ability to sequestrate U(VI) from aqueous solutions. As a result, MIL-100(Al) performed the best among the tested...

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A ternary mechanism for the facilitated transfer of metal ions onto metal-organic frameworks: implications for the ''versatility'' of these materials as solid sorbents

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