Oxidative degradation of p-chlorophenol by the persulfate-doped Fe–Mn bimetallic hydroxide, the parametrical significance, and systematical optimization
[Yu, Danni; Deng, Shihan; Liu, Longfei; Du, Jing; Huang, Tao] Changshu Inst Technol, Sch Mat Engn, Changshu 215500, Jiangsu, Peoples R China.
[Zhang, Shuwen] Univ South China, Nucl Resources Engn Coll, Hengyang 421001, Hunan, Peoples R China.
通讯机构:
[Tao Huang; Jing Du] S
School of Materials Engineering, Changshu Institute of Technology, Changshu, China<&wdkj&>School of Materials Engineering, Changshu Institute of Technology, Changshu, China
This study received funding from The China Postdoctoral Science Foundation (2020M681774), the Natural Science Foundation of the Jiangsu Higher Education Institutions of China (20KJB490001), and Xuzhou Science and Technology Bureau (Nos. KC19228 and KC20055).
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院系归属:
核资源工程学院
摘要:
Aqueous Fe(II)-catalyzed activation commonly deteriorates the oxidation performance of persulfate (PS) to the treatment of organic contaminants. In this study, a PS-doped layered bimetallic hydroxide (Fe–Mn hydroxide) was synthesized to construct a heterogeneously catalytic system to solve the issue brought by homogeneity. The molar ratio of Fe(II) to Mn(II) and the mass ratio of PS to Fe–Mn hydroxide both had a significant impact on the catalytic degradation of p-CP. Reaction temperatures engaged in the most essential role in influencing the...