A method was established to quantitatively estimate sources of atmospheric carbonaceous matter, using a combination of radiocarbon technology, linear regression of organic carbon (OC) -K+ and elemental carbon (EC) tracer method. Fractional contributions of fossil fuels, biomass burning, biogenic secondary organic carbon (BSOC) and soil dust to the atmospheric size-resolved carbonaceous matters in Shanghai suburb were estimated using this new method. The fossil carbon contributed most of the OC in particles smaller than 0.49 μm, and its fractio...