Unraveling complexation and enantioseparation of a new chiral-at-uranium complex to chiral pesticides R/S-malaoxons

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成果类型：

期刊论文

作者：

Guo, Meng-zhen;Ouyang, Wen-jun;Wang, Yun;Kong, Xiang-he;Xiao, Xi-lin;...

通讯作者：

Nie, Chang-ming;Peng, GW

作者机构：

[Peng, Guo-wen; Guo, Meng-zhen; Xiao, Xi-lin; Wang, Yun; Kong, Xiang-he; Nie, Chang-ming; Ouyang, Wen-jun] Univ South China, Sch Chem & Chem Engn, Hengyang, Peoples R China.

[Peng, Guo-wen; Guo, Meng-zhen; Xiao, Xi-lin; Wang, Yun; Kong, Xiang-he; Nie, Chang-ming; Ouyang, Wen-jun] Theoret Res Dept, Key Lab Hunan Prov Design & Applicat Nat Actinide, Hengyang, Peoples R China.

[Peng, Guo-wen; Peng, GW; Nie, Chang-ming; Nie, CM] Theoret Res Dept, Key Lab Hunan Prov Design & Applicat Nat Actinide, Hengyang 421001, Peoples R China.

通讯机构：

[Peng, GW ; Nie, CM] T

Theoret Res Dept, Key Lab Hunan Prov Design & Applicat Nat Actinide, Hengyang 421001, Peoples R China.

语种：

英文

关键词：

chiral pesticides;chiral-at-uranium complex;density functional theory (DFT);enantioseparation;R/S-malaoxons

期刊：

Applied Organometallic Chemistry

ISSN：

0268-2605

年：

2024

卷：

期：

DOI：

10.1002/aoc.7428

基金类别：

National Natural Science Foundation of China; Hunan Provincial Natural Science Foundation of China [2020JJ6049]; University of South China; [42377076]

机构署名：

本校为第一机构

院系归属：

化学化工学院

摘要：

Unraveling uranium complexes has become a popular study topic in recent years to address the problem of spent fuel treatment. An important and promising investigation is the enantiomer separation of chiral organophosphorus pesticides (OPs) via uranyl-containing receptors. Among them, malaoxon (MLX), as a chiral OP with high toxicity and good selectivity, is controversial because of the different toxicity differences caused by the R and S configurations to target and non-target organisms. Therefore, it is crucial to explore effective methods for separating its enantiomers. In this work, a novel...

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Unraveling complexation and enantioseparation of a new chiral-at-uranium complex to chiral pesticides R/S-malaoxons

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