Regulating Polymeric Adsorption Dynamics via Monolayer-Architected Hydrotalcite Integration for High-Performance Organic Solar Cells

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成果类型：

期刊论文

作者：

Li, Zhenye;Ding, Xu;Jiang, Dongcheng;Ding, Yu-Feng;Liu, Biao;...

通讯作者：

Yin, H;Ding, YF;Zeng, DQ

作者机构：

[Li, Zhenye; Ding, Xu] Univ South China, Coll Mech Engn, Hengyang 421001, Peoples R China.

[Yin, H; Yin, Hang; Jiang, Dongcheng] Shandong Univ, Sch Phys, State Key Lab Crystal Mat, Jinan 250100, Peoples R China.

[Ding, YF; Ding, Yu-Feng] Univ South China, Sch Math & Phys, Hengyang 421001, Peoples R China.

[Liu, Biao] Cent South Univ, Sch Phys & Elect, Changsha 410083, Peoples R China.

[Zhao, Yu-Qing] Hunan Univ Sci & Technol, Sch Phys & Elect Sci, Xiangtan 411201, Peoples R China.

通讯机构：

[Yin, H ] S

[Ding, YF ; Zeng, DQ ] U

Shandong Univ, Sch Phys, State Key Lab Crystal Mat, Jinan 250100, Peoples R China.

Univ South China, Sch Math & Phys, Hengyang 421001, Peoples R China.

Univ South China, Sch Nucl Sci & Technol, Hengyang 421001, Peoples R China.

语种：

英文

关键词：

hydrotalcite;molecular aggregation;organic solar cells;polymer donor

期刊：

Advanced Materials

ISSN：

0935-9648

年：

2025

卷：

期：

页码：

e2508049

DOI：

10.1002/adma.202508049

基金类别：

National Natural Science Foundation of China [62404094/12204272]; National Natural Science Foundation of China (NSFC) [2023JJ40532]; Natural Science Foundation of Hunan Province [210XQD018]; Fund of University of South China [202121014588]; Fund of Hengyang Science and Technology Bureau

机构署名：

本校为第一且通讯机构

院系归属：

机械工程学院

核科学技术学院

数理学院

摘要：

In organic solar cells (OSCs), the molecular aggregation property of donor-acceptor bulk heterojunction (BHJ) architectures serves as a critical determinant in device performance. Nevertheless, the intrinsic steric constraints imposed by polymeric side chains frequently lead to metastable molecular packing configurations with diminished structural coherence. In this study, a morphological modulation strategy is proposed by adopting a 2D layered hydrotalcite (HDC) nanocrystal to regulate polymeric adsorption dynamics. By leveraging hydroxyl-dire...

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Regulating Polymeric Adsorption Dynamics via Monolayer-Architected Hydrotalcite Integration for High-Performance Organic Solar Cells

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