3D/2D MnO/MXene heterostructure with high efficiency for adsorbing uranium

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成果类型：

期刊论文

作者：

Zhang, Chao;Wang, Yi;Liu, Yi-Lin*;Zeng, Qingming;Wen, Yanjun;...

通讯作者：

Liu, Yi-Lin;Zeng, QY

作者机构：

[Chen, Haodong; Liu, Yi-Lin; Zeng, Qingyi; Liu, YL; Zhang, Chao; Xie, Xinyi; Guo, Lulin; Wen, Yanjun; Zeng, Qingming] Univ South China, Sch Mech Engn, Hengyang 421001, Peoples R China.

[Chen, Haodong; Liu, Yi-Lin; Zeng, Qingyi; Liu, YL; Zhang, Chao; Xie, Xinyi; Guo, Lulin; Wen, Yanjun; Zeng, Qingming] Univ South China, Sch Resources & Environm & Safety Engn, Hengyang 421001, Peoples R China.

[Wang, Yi] Tsinghua Univ, Lab Environm Technol, INET, Beijing 100084, Peoples R China.

通讯机构：

[Zeng, QY ; Liu, YL] U

Univ South China, Sch Mech Engn, Hengyang 421001, Peoples R China.

Univ South China, Sch Resources & Environm & Safety Engn, Hengyang 421001, Peoples R China.

语种：

英文

关键词：

MnO nanosheet;MXene;Uranium adsorption;Surface oxygen groups;Chemisorption

期刊：

Chemical Engineering Journal

ISSN：

1385-8947

年：

2024

卷：

485

页码：

149856

DOI：

10.1016/j.cej.2024.149856

基金类别：

CRediT authorship contribution statement Chao Zhang: Writing – original draft, Software, Methodology, Investigation. Yi Wang: Writing – review & editing, Methodology. Yi-Lin Liu: Writing – review & editing, Methodology, acquisition, Conceptualization. Qingming Zeng: Software, Investigation. Yanjun Wen: Visualization, Software. Lulin Guo: Investigation. Haodong Chen: Investigation. Xinyi Xie: Visualization. Qingyi Zeng: Writing – review & editing, Supervision, Project administration, acquisition, Data curation,

机构署名：

本校为第一且通讯机构

院系归属：

机械工程学院

摘要：

An innovative MnO/Ti3C2 MXene heterostructure, consisting of three-dimensional (3D) MnO nanosheet array directly assembled on two-dimensional (2D) Ti3C2 MXene nanosheets, was synthesized via a simple hydrothermal-annealing strategy for uranium elimination. This unique 3D/2D heterostructure derived substantially high specific surface area (311.9 m2/g) and exposed considerable amount of surface oxygen groups, including surface lattice M-O and adsorbed -OH. Through a comprehensive exploration encompassing adsorbent dosage, pH, ionic strength, initial U(VI) concentration, and environmental conditi...

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3D/2D MnO/MXene heterostructure with high efficiency for adsorbing uranium

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