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Single Nanoparticle to 3D Supercage: Framing for an Artificial Enzyme System

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成果类型:
期刊论文
作者:
Cai, Ren;Yang, Dan;Peng, Shengjie;Chen, Xigao;Huang, Yun;...
通讯作者:
Tan, Weihong
作者机构:
[Yang, Shengyuan; Liu, Yuan; Liu, Zhenbao; Chen, Xigao; Hou, Weijia; Huang, Yun; Cai, Ren; Tan, Weihong] Univ Florida, Dept Chem, Ctr Res Bio Nano Interface, Gainesville, FL 32611 USA.
[Yang, Shengyuan; Liu, Yuan; Liu, Zhenbao; Chen, Xigao; Hou, Weijia; Huang, Yun; Cai, Ren; Tan, Weihong] Univ Florida, UF Genet Inst, Hlth Canc Ctr, Dept Physiol & Funct Genom, Gainesville, FL 32611 USA.
[Yang, Shengyuan; Liu, Yuan; Liu, Zhenbao; Chen, Xigao; Hou, Weijia; Huang, Yun; Cai, Ren; Tan, Weihong] Univ Florida, McKnight Brain Inst, Gainesville, FL 32611 USA.
[Tan, Weihong] Hunan Univ, Coll Biol, Coll Chem & Chem Engn, Mol Sci & Biomed Lab,State Key Lab Chemo Bio Sen, Changsha 410082, Hunan, Peoples R China.
[Tan, Weihong] Hunan Univ, Collaborat Res Ctr Mol Engn Theranost, Changsha 410082, Hunan, Peoples R China.
通讯机构:
[Tan, Weihong] U
Univ Florida, Dept Chem, Ctr Res Bio Nano Interface, Gainesville, FL 32611 USA.
语种:
英文
期刊:
Journal of the American Chemical Society
ISSN:
0002-7863
年:
2015
卷:
137
期:
43
页码:
13957-13963
基金类别:
National Institutes of HealthUnited States Department of Health & Human ServicesNational Institutes of Health (NIH) - USA [GM079359, GM111386, CA133086]; National Key Scientific Program of China [2011CB911000]; NSFC grantsNational Natural Science Foundation of China (NSFC) [NSFC 21221003, NSFC 21327009]; China National Instrumentation Program [2011YQ03012412]; NATIONAL CANCER INSTITUTEUnited States Department of Health & Human ServicesNational Institutes of Health (NIH) - USANIH National Cancer Institute (NCI) [R01CA133086, R01CA133086, R01CA133086, R01CA133086, R01CA133086] Funding Source: NIH RePORTER; NATIONAL INSTITUTE OF GENERAL MEDICAL SCIENCESUnited States Department of Health & Human ServicesNational Institutes of Health (NIH) - USANIH National Institute of General Medical Sciences (NIGMS) [R01GM079359, R01GM079359, R01GM079359, R01GM079359, R01GM079359, R01GM079359, R01GM079359, R01GM111386, R01GM079359, R01GM111386, R01GM079359, R01GM111386] Funding Source: NIH RePORTER
机构署名:
本校为其他机构
院系归属:
公共卫生学院
摘要:
A facile strategy has been developed to fabricate Cu(OH)2 supercages (SCs) as an artificial enzyme system with intrinsic peroxidase-mimic activities (PMA). SCs with high catalytic activity and excellent recyclability were generated via direct conversion of amorphous Cu(OH)2 nanoparticles (NPs) at room temperature. More specifically, the process that takes a single nanoparticle to a 3D supercage involves two basic steps. First, with addition of a copper-ammonia complex, the Cu2+ ions that are located on the surface of amorphous Cu(OH)2 NPs would...

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