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Fe-N-coordinated graphene-like honeycomb porous carbon as an extremely effective catalyst for catalytic oxidation

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成果类型:
期刊论文
作者:
Wu, Meiling;Tao, Yang;Liu, Yuwei;Hou, Sanying*;Xiao, Tiyang;...
通讯作者:
Hou, Sanying;Shi, L;Peng, GW
作者机构:
[Wu, Meiling; Liu, Yuwei; Shi, Lang; Shi, L; Hou, Sanying; Xiao, Tiyang; Fu, Qing] Univ South China, Sch Chem & Chem Engn, Hengyang 421001, Peoples R China.
[Tao, Yang; Peng, Guowen] Univ South China, Sch Resource Environm & Safety Engn, Hengyang 421001, Peoples R China.
通讯机构:
[Shi, L ; Hou, SY; Peng, GW ] U
Univ South China, Sch Chem & Chem Engn, Hengyang 421001, Peoples R China.
Univ South China, Sch Resource Environm & Safety Engn, Hengyang 421001, Peoples R China.
语种:
英文
关键词:
Honeycomb porous carbon;Fe-NC;PMS;Tetracycline;Superoxide radical
期刊:
Separation and Purification Technology
ISSN:
1383-5866
年:
2025
卷:
354
页码:
129225
基金类别:
National Natural Science Foundation of China [22109068]; Undergraduate Innovation and Entrepreneurship of China [S202310555072]
机构署名:
本校为第一且通讯机构
院系归属:
化学化工学院
摘要:
In this study, Fe/N co-doped graphene-like honeycomb porous carbon (Fe-NC)was produced and used for the activating PMS to degrade TC. The Fe-NC catalyst has shown high activity in the TC degradation by activated PMS, with an efficiency of up to 94 % in 30 min. while the blank catalyst without N and Fe doping exhibited the lowest performance with 47.3 % TC degradation. Moreover, other operational factors of Fe-NC catalysts were also investigated to evaluate its catalytic activity. The burst experiments and electron paramagnetic resonance (EPR) experiments demonstrated that free radical paths (O...

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