Monolayer MnPS3 Nanosheet Integration for Extended Exciton Diffusion and Charge Transport in High-Performance Thickness-Insensitive Organic Photovoltaics

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成果类型：

期刊论文

作者：

Li, Zhenye;Zhou, Rujin;Su, Zhaoxiong;Mao, Min;Li, Zhijun;...

通讯作者：

Li, ZY;Zeng, DQ;Lai, HJ

作者机构：

[Li, Zhijun; Su, Zhaoxiong; Li, Zhenye; Zhou, Rujin; Mao, Min] Univ South China, Coll Mech Engn, Hengyang 421001, Peoples R China.

[Zeng, Deqian] Univ South China, Sch Nucl Sci & Technol, Hengyang 421001, Peoples R China.

[Zhu, Chunguang] Sichuan Univ Sci & Engn, Sch Mat Sci & Engn, Zigong 643002, Sichuan, Peoples R China.

[Lai, Hanjian] Univ South China, Sch Elect Engn, Hengyang 421001, Peoples R China.

通讯机构：

[Li, ZY ; Lai, HJ ; Zeng, DQ ] U

Univ South China, Coll Mech Engn, Hengyang 421001, Peoples R China.

Univ South China, Sch Nucl Sci & Technol, Hengyang 421001, Peoples R China.

Univ South China, Sch Elect Engn, Hengyang 421001, Peoples R China.

语种：

英文

关键词：

charge transport;exciton diffusion;monolayer MnPS3 nanosheet;organic photovoltaics;thickness-insensitive

期刊：

Advanced Materials

ISSN：

0935-9648

年：

2025

页码：

e13125

DOI：

10.1002/adma.202513125

基金类别：

Fund of Hengyang Science and Technology Bureau

机构署名：

本校为第一且通讯机构

院系归属：

机械工程学院

电气工程学院

核科学技术学院

摘要：

Industrial-scale roll-to-roll processing of organic photovoltaics (OPVs) requires photoactive layers ≥300 nm for manufacturability and mechanical robustness, yet state-of-the-art high-efficiency systems remain confined to 80-120 nm due to intrinsic exciton diffusion and charge transport limitations. To resolve this fundamental thickness-efficiency trade-off, monolayer MnPS(3) nanosheet (1-2 nm) via liquid-phase exfoliation are engineered to extend exciton diffusion lengths and out-of-plane charge mobility, as validated through multimodal chara...

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Monolayer MnPS3 Nanosheet Integration for Extended Exciton Diffusion and Charge Transport in High-Performance Thickness-Insensitive Organic Photovoltaics

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