期刊论文

Wu, Sheng-Tao;Lin, YW;Wang, H

英文

Biosensors and Bioelectronics

0956-5663

2024

263

116580

10.1016/j.bios.2024.116580

CRediT authorship contribution statement Sheng-Tao Wu: Writing – review & editing, Writing – original draft, Supervision, Conceptualization. Zhi-Yu Qiu: Methodology, Investigation, Formal analysis, Data curation. Hui-Qi Su: Project administration, Methodology. Ying Cao: Investigation, acquisition. Shu-Qin Gao: Resources, Methodology. Hui Wang: Visualization, Supervision, Methodology, Data curation. Cong-Hui Wang: Visualization, Methodology, Formal analysis. Ying-Wu Lin: Writing – review & editing, Visualization, Validation,

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A Mn-based nanozyme, Mn-uNF/Si, with excellent alkali phosphatase-like activity was designed by in-situ growth of ultrathin Mn-MOF on the surface of silicon spheres, and implemented as an effective solid Lewis-Brønsted acid catalyst for broad-spectrum dephosphorylation. H(2)(18)O-mediated GC-MS studies confirmed the cleavage sites and the involvement of H(2)O in the new bonds. DRIFT NH(3)-IR and in-situ ATR-FTIR confirmed the coexistence of Lewis-Brønsted acid sites and the adjustment of adsorption configurations at the interfacial sites. In ...