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A new strategy to construct MOF-on-MOF derivatives for the removal of tetracycline hydrochloride from water by activation of peroxymonosulfate

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成果类型:
期刊论文
作者:
Fengtao Hu;Shunyan Ning*;Zengzhiqiang Li;Hao Zhu;Toyohisa Fujita;...
通讯作者:
Shunyan Ning
作者机构:
[Toyohisa Fujita; Zengzhiqiang Li; Fengtao Hu; Hao Zhu] State Key Laboratory of Featured Metal Materials and Life-cycle Safety for Composite Structures, MOE Key Laboratory of New Processing Technology for Nonferrous Metals and Materials, School of Resources, Environment and Materials, Guangxi University, Nanning, 530004, China
[Shunyan Ning] School of Nuclear Science and Technology, University of South China, 28 Changsheng West Road, Hengyang, 421001, China. Electronic address: ningshunyan@usc.edu.cn
[Deqian Zeng; Yuezhou Wei; Mohammed F. Hamza; Xiangbiao Yin; Lifeng Chen] School of Nuclear Science and Technology, University of South China, 28 Changsheng West Road, Hengyang, 421001, China
[Yuezhou Wei] School of Nuclear Science and Engineering, Shanghai Jiao Tong University, 800 Dong Chuan Road, Shanghai, 200240, China
[Xinpeng Wang] State Key Laboratory of Featured Metal Materials and Life-cycle Safety for Composite Structures, MOE Key Laboratory of New Processing Technology for Nonferrous Metals and Materials, School of Resources, Environment and Materials, Guangxi University, Nanning, 530004, China. Electronic address: wangxinpeng@gxu.edu.cn
通讯机构:
[Shunyan Ning] S
School of Nuclear Science and Technology, University of South China, 28 Changsheng West Road, Hengyang, 421001, China
语种:
英文
关键词:
Advanced oxidative process;Fukui function;MOF derivative;Peroxymonosulfate;Tetracycline
期刊:
Chemosphere
ISSN:
0045-6535
年:
2024
卷:
362
页码:
142676
基金类别:
CRediT authorship contribution statement Fengtao Hu: Writing – original draft, Methodology, Data curation. Shunyan Ning: Writing – review & editing, acquisition. Zengzhiqiang Li: Investigation. Hao Zhu: Investigation. Toyohisa Fujita: Supervision. Xiangbiao Yin: Methodology. Lifeng Chen: Methodology. Deqian Zeng: Methodology. Mohammed F. Hamza: Supervision. Yuezhou Wei: Validation. Xinpeng Wang: Project administration.
机构署名:
本校为通讯机构
院系归属:
核科学技术学院
摘要:
A MOF-on-MOF composite derivative material named ZIF-67@Ce-MOF-600 was designed and synthesized. The preparation of ZIF-67@Ce-MOF-600 was optimized from the aspects of the ratio of metal and ligand, heat-treatment temperature. It was demonstrated by XRD, FT-IR, SEM-EDS and TEM. The optimum conditions for the activation of PMS by ZIF-67@Ce-MOF-600 for the degradation of tetracycline (TC) were investigated by adjusting the catalyst dosage, TC, pH, peoxymonosulfate (PMS) concentration, and different kinds of water, co-existing anions and pollution. Under optimal conditions (20 mg catalysts and 50...

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