Hydrogen bonding-tuned hydroxo-bridged tetra-copper Cu4(bipy)4-cluster supramolecular network to layered coordination polymer

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期刊论文

作者：

Zhang, Jian;Chen, Yang-Yang;Tan, Chunhong*;Ma, Xiao*;Wang, Xiao-Feng*;...

通讯作者：

Tan, Chunhong;Wang, Xiao-Feng;Ma, Xiao

作者机构：

[Chen, Yang-Yang; Tan, Chunhong; Wang, Xiao-Feng; Zhang, Jian] Univ South China, Sch Chem & Chem Engn, Hengyang 421001, Peoples R China.

[Ma, Xiao] Changzhou Univ, Sch Petrochem Engn, Adv Catalysis & Green Mfg Collaborat Innovat Ctr, Jiangsu Key Lab Adv Catalyt Mat & Technol, Changzhou 213164, Jiangsu, Peoples R China.

[Wang, Xiao-Feng] Univ South China, Hunan Key Lab Design & Applicat Actinide Complexe, Hengyang 421001, Peoples R China.

[Ou, Guangchuan] Hunan Univ Sci & Engn, Dept Biol & Chem, Yongzhou 425199, Peoples R China.

通讯机构：

[Tan, CH; Wang, XF; Wang, Xiao-Feng] U

[Ma, Xiao] C

Univ South China, Sch Chem & Chem Engn, Hengyang 421001, Peoples R China.

Changzhou Univ, Sch Petrochem Engn, Adv Catalysis & Green Mfg Collaborat Innovat Ctr, Jiangsu Key Lab Adv Catalyt Mat & Technol, Changzhou 213164, Jiangsu, Peoples R China.

Univ South China, Hunan Key Lab Design & Applicat Actinide Complexe, Hengyang 421001, Peoples R China.

语种：

英文

期刊：

CrystEngComm

ISSN：

1466-8033

年：

2020

卷：

期：

页码：

5255-5262

DOI：

10.1039/d0ce00985g

基金类别：

National Science Foundation of ChinaNational Natural Science Foundation of China (NSFC) [11375082, 51772091, 21701081]; Hunan Provincial Natural Science Foundation of ChinaNatural Science Foundation of Hunan Province [2020JJ5473]; Natural Science Foundation of Jiangsu ProvinceJiangsu Planned Projects for Postdoctoral Research FundsNatural Science Foundation of Jiangsu Province [BK20170290]

机构署名：

本校为第一且通讯机构

院系归属：

化学化工学院

摘要：

Three tetranuclear Cu(ii) coordination compounds have been synthesized by the self-assembly of copper(ii) nitrate with N/O donating bi-ligands through ammonia aqueous/ethanol mixture solution reaction. Single crystal structural analyses have shown that the three compounds feature chair-like hydroxo-bridged tetra-copper(ii) cluster: symmetric [Cu4(bipy)4(OH)4(H2O)2]4+ in 1, asymmetric [Cu4(bipy)4(OH)4(H2O)(1,3-DBC)]2+ in 2, and symmetric [Cu4(bipy)4(OH)2(1,2-BDC)2]2+ in 3 (bipy = 2,2′-bipyridineand H2BDC = benzene dicarboxylic acid). Three bito...

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Hydrogen bonding-tuned hydroxo-bridged tetra-copper Cu4(bipy)4-cluster supramolecular network to layered coordination polymer

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