Cold sintering of ammonium phosphomolybdate ((NH4)3PMo12O40·xH2O) as soild-state matrices for cesium immobilization

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成果类型：

期刊论文

作者：

Zhang, Chi;Chen, Pengju*;Zhou, Yi;Ji, Yue;Ning, Shunyan;...

通讯作者：

Chen, Pengju;Yin, XB

作者机构：

[Ji, Yue; Yin, Xiangbiao; Chen, Pengju; Ning, Shunyan; Wei, Yuezhou; Zhang, Chi; Zhou, Yi; Chen, Lifeng] Univ South China, Sch Nucl Sci & Technol, 28 Changsheng West Rd, Hengyang 421001, Peoples R China.

[Xie, Yupeng] Univ South China, Sch Resource Environm & Safety Engn, 28 Changsheng West Rd, Hengyang 421001, Peoples R China.

[Wu, Hao; Wei, Yuezhou; Wu, Yan] Shanghai Jiao Tong Univ, Sch Nucl Sci & Engn, 800 Dong Chuan Rd, Shanghai 200240, Peoples R China.

[Shi, Weiqun] Chinese Acad Sci, Inst High Energy Phys, Lab Nucl Energy Chem, 19B Yuquan Rd, Beijing 100049, Peoples R China.

[Yin, Xiangbiao] Univ South China, Key Lab Adv Nucl Energy Design & Safety, Minist Educ, 28 Changsheng West Rd, Hengyang, Peoples R China.

通讯机构：

[Yin, XB ; Chen, PJ] U

Univ South China, Sch Nucl Sci & Technol, 28 Changsheng West Rd, Hengyang 421001, Peoples R China.

语种：

英文

关键词：

Cold sintering process;Cs-adsorbed APM;Solidification;Densification;Cs immobilization mechanism

期刊：

Journal of Environmental Management

ISSN：

0301-4797

年：

2025

卷：

382

页码：

125232

DOI：

10.1016/j.jenvman.2025.125232

基金类别：

National Natural Science Foundation of China [22206073, 22350710186, U23B20167]; Scientific Research Program of FuRong Laboratory [2023SK2098]

机构署名：

本校为第一且通讯机构

院系归属：

核科学技术学院

摘要：

Ammonium phosphomolybdate (APM) is often used for the adsorption of Cs + . However, the decomposition temperature of cesium-containing ammonium phosphomolybdate waste is low and difficult to dispose of. This study introduces the first use of cold sintering to solidify ammonium phosphomolybdate monomers at low temperatures. The maximum adsorption capacity of the synthesized ammonium phosphomolybdate was 112.58 mg/g. Cold sintering results indicate that the HNO 3 was more effective than other acidic or salt solutions for densifying ammonium phosp...

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Cold sintering of ammonium phosphomolybdate ((NH4)3PMo12O40·xH2O) as soild-state matrices for cesium immobilization

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