Architecture of CoNx single clusters on nanocarbon as excellent oxygen reduction catalysts with high-efficient atomic utilization

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期刊论文

作者：

He, Ting;Xue, Hui;Wang, Xiaojuan;He, Shuanghua;Lei, Yulai;...

通讯作者：

Zhang, Yi;Xiang, Juan

作者机构：

[Xue, Hui; He, Ting; Lei, Yulai; Zhang, Y; Xiang, Juan; Zhang, Yi; Wang, Xiaojuan; Zhang, Yuyuan] Cent S Univ, Hunan Prov Key Lab Efficient & Clean Utilizat Man, Coll Chem & Chem Engn, 932 Lushan South Rd, Changsha, Hunan, Peoples R China.

[Wang, Xiaojuan] Univ South China, Coll Chem & Chem Engn, Hengyang, Hunan, Peoples R China.

[He, Shuanghua] Hefei Univ Technol, Sch Mech Engn, Hefei 230009, Peoples R China.

[Shen, Rujuan] Cent S Univ, State Key Lab Power Met, 932 Lushan South Rd, Changsha, Hunan, Peoples R China.

通讯机构：

[Zhang, Y; Xiang, J] C

Cent S Univ, Hunan Prov Key Lab Efficient & Clean Utilizat Man, Coll Chem & Chem Engn, 932 Lushan South Rd, Changsha, Hunan, Peoples R China.

语种：

英文

期刊：

Nanoscale

ISSN：

2040-3364

年：

2017

卷：

期：

页码：

8341-8348

DOI：

10.1039/c7nr02165h

基金类别：

National Nature Science Foundation of ChinaNational Natural Science Foundation of China (NSFC) [21473257]; National High Technology Research and Development Program of ChinaNational High Technology Research and Development Program of China [2015AA020502]; Tian Shan scholar program of Xinjiang University; Fundamental Research Funds for the Central Universities of Central South University [502220001]; Hunan Provincial Science and Technology Plan Project of China [2016TP1007]; Open-End Fund for the Valuable and Precision Instruments of Central South University; High Performance Computing Center of Central South University, China; State Key Laboratory of Powder Metallurgy, Central South University

机构署名：

本校为其他机构

院系归属：

化学化工学院

摘要：

A new strategy to fabricate CoNxsingle cluster supported nanocarbon catalysts (C/P/2Co600) with enhanced atomic utilization towards the oxygen reduction reaction (ORR) is reported. N-Coordination protection and low-temperature pyrolysis are the two key factors for the formation of CoNxsingle clusters on nanocarbon supports. Morphological and structural identification confirmed the simultaneous anchoring of homo-dispersed CoNxsingle clusters and N-doping on the nanocarbon under relatively mild thermal treatment conditions. Expectedly, the obtained single cluster catalyst with a trace amount of ...

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Architecture of CoNx single clusters on nanocarbon as excellent oxygen reduction catalysts with high-efficient atomic utilization

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