Ambient N2 Reduction to NH3 Electrocatalyzed by ZIF-67-Derived Nitrogen-Doped Porous Carbon Supported Co9S8 Nanomaterials - 成果

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Ambient N₂ Reduction to NH₃ Electrocatalyzed by ZIF-67-Derived Nitrogen-Doped Porous Carbon Supported Co₉S₈ Nanomaterials

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成果类型：

期刊论文

作者：

Zhang, Huanhuan;Yan, Shuhao;Yi, Wei;Ma, Xiao;He, Jing;...

通讯作者：

Yi, LH;Lu, YB;Wang, XZ;Yi, W

作者机构：

[Yi, Lanhua; Yi, LH; He, Jing; Zhang, Huanhuan; Ma, Xiao] Xiangtan Univ, Sch Chem, Key Lab Environmentally Friendly Chem & Applicat, Minist Educ, Xiangtan 411105, Peoples R China.

[Lu, Yebo; Lu, YB] Jiaxing Univ, Coll Informat Sci & Engn, Jiaxing 314001, Peoples R China.

[Wang, Xingzhu; Wang, XZ] Univ South China, Sch Elect Engn, Hengyang 421001, Peoples R China.

[Yi, Wei; Yi, W] Minzu Normal Univ Xingyi, Sch Biol & Chem, Xingyi 562400, Peoples R China.

[Yan, Shuhao] Natl Ctr Nanosci & Technol, Beijing 100190, Peoples R China.

通讯机构：

[Yi, LH ] X

[Lu, YB ] J

[Yi, W ] M

[Wang, XZ ] U

Xiangtan Univ, Sch Chem, Key Lab Environmentally Friendly Chem & Applicat, Minist Educ, Xiangtan 411105, Peoples R China.

语种：

英文

关键词：

Co9S8 composite nanocatalyst;electrocatalytic nitrogenreduction reaction;NH3 yield rate;Faradaicefficiency

期刊：

ACS SUSTAINABLE CHEMISTRY & ENGINEERING

ISSN：

2168-0485

年：

2024

DOI：

10.1021/acssuschemeng.3c08087

基金类别：

Department of Education of Guizhou Province [52371237]; National Natural Science Foundation of China [2023JJ50287, 2023JJ50132]; Natural Science Foundation of Hunan Province, China [2022396]; Scientific Research Project of Colleges and Universities of the Guizhou Provincial Education Department [2022-1-20]; Science and Technology Planning Project of the Science and Technology Bureau of Qianxinan Prefecture [23XYBS19]; Doctoral Research Start-up Fund of Minzu Normal University of Xingyi

机构署名：

本校为通讯机构

院系归属：

电气工程学院

摘要：

The electrocatalytic nitrogen reduction reaction (eNRR) under ambient conditions is a promising alternative to the Haber-Bosch process, but one of the primary pending issues for the eNRR is the development of efficient and stable electrocatalysts. Herein, we propose to prepare a ZIF-67-derived nitrogen-doped porous carbon-supported Co9S8 nanocomposite achieving the maximum average of 9.80 mu g h(-1) mg(cat)(-1) NH3 yield and the highest Faradaic efficiency (FE) of 9.89% in 0.1 M Na2SO4. Moreover, Co9S8/NC shows excel...

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Ambient N₂ Reduction to NH₃ Electrocatalyzed by ZIF-67-Derived Nitrogen-Doped Porous Carbon Supported Co₉S₈ Nanomaterials

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