To understand the physical and chemical characteristics, particle size distribution and sources of size-separated aerosols in Lhasa, which is located on the Tibetan Plateau (TP), six sizes of aerosol samples were collected in Lhasa in 2014. Ca(2+), NH4(+), NO3(-), SO4(2-) and Cl(-) were the dominant ions. The ratio of cation equivalents (CE) to anion equivalents (AE) for each particle size segment indicated that the atmospheric aerosols in Lhasa were alkaline. SO4(2-) and NO3(-) could be neutralized by Ca(2+), but could not be neutralized by NH4(+), according to the [NH4(+)]/[NO3(-)+SO4(2-)] a...