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ENGINEERING MULTILEVEL COLLABORATIVE CATALYTIC INTERFACES WITH MULTIFUNCTIONAL IRON SITES ENABLING HIGH-PERFORMANCE REAL SEAWATER SPLITTING

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成果类型:
期刊论文
作者:
Zhang, Fangming;Liu, Yilin;Yu, Fang;Pang, Hongjing;Zhou, Xuan;...
通讯作者:
Fang Yu<&wdkj&>Haiqing Zhou
作者机构:
[Zhang, Fangming; Li, Dongyang; Pang, Hongjing; Zhou, Qian; Zhou, Haiqing; Zhou, Xuan; Ma, Wenqi; Yu, Fang] Hunan Normal Univ, Dept Phys, Key Lab Matter Microstruct & Funct Hunan Prov, Key Lab Low Dimens Quantum Struct & Quantum Contro, Changsha 410081, Peoples R China.
[Zhang, Fangming; Li, Dongyang; Pang, Hongjing; Zhou, Qian; Zhou, Haiqing; Zhou, Xuan; Ma, Wenqi; Yu, Fang] Hunan Normal Univ, Synerget Innovat Ctr Quantum Effects & Applicat, Changsha 410081, Peoples R China.
[Liu, Yilin] Univ South China, Sch Mech Engn, Hengyang 421001, Peoples R China.
[Mo, Yuxue] Hengyang Normal Univ, Coll Phys & Elect Engn, Hengyang 421002, Peoples R China.
通讯机构:
[Fang Yu; Haiqing Zhou] K
Key Laboratory of Low-Dimensional Quantum Structures and Quantum Control of Ministry of Education, Key Laboratory for Matter Microstructure and Function of Hunan Province, Department of Physics and Synergetic Innovation Center for Quantum Effects and Applications, Hunan Normal University, Changsha 410081, China
语种:
英文
关键词:
seawater splitting;electrocatalyst;bifunctional water splitting;non-noble metal;porous material
期刊:
ACS Nano
ISSN:
1936-0851
年:
2023
卷:
17
期:
2
页码:
1681-1692
基金类别:
National Science Foundation of China [52172197]; Youth 1000 Talent Program of China, Science and Technology Innovation Platform [2019RS1032]; Major Projects "Takes the Lead" of Natural Science Foundation; Undergraduate Scientific Research Innovation Project of Hunan Province [2021JC0008, 2022213]; Hunan Normal University [22CSZ011, 22CSZ010, 22CSY156]
机构署名:
本校为其他机构
院系归属:
机械工程学院
摘要:
Given the abundant reserves of seawater and the scarcity of freshwater, real seawater electrolysis is a more economically appealing technology for hydrogen production relative to orthodox freshwater electrolysis. However, this technology is greatly precluded by the undesirable chlorine oxidation reaction and severe chloride corrosion at the anode, further restricting the catalytic efficiency of overall seawater splitting. Herein, a feasible strategy by engineering multifunctional collaborative catalytic interfaces is reported to develop porous metal nitride/phosphide heterostructure arrays anc...

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