Lewis Acid-Assisted Molybdenum(VI) Complexes with S, N-bidentate Ligands to Reduce Nitrate

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成果类型：

期刊论文

作者：

Lang, Jia-Jia;Mi, Pengbing;Wang, Xiao-Juan;Gao, Shu-Qin;Tan, Xiangshi;...

通讯作者：

Dr. Pengbing Mi<&wdkj&>Prof. Dr. Ying-Wu Lin<&wdkj&>Dr. Pengbing Mi Dr. Pengbing Mi Dr. Pengbing Mi<&wdkj&>Prof. Dr. Ying-Wu Lin Prof. Dr. Ying-Wu Lin Prof. Dr. Ying-Wu Lin

作者机构：

[Lang, Jia-Jia; Lin, Ying-Wu] Univ South China, Sch Chem & Chem Engn, Hengyang Med Coll, Hengyang 421001, Peoples R China.

[Mi, Pengbing] Univ South China, Dept Pharm, Hengyang Med Sch, Hengyang 421001, Hunan, Peoples R China.

[Gao, Shu-Qin; Lin, Ying-Wu; Wang, Xiao-Juan] Univ South China, Key Lab Prot Struct & Funct Univ Hunan Prov, Hengyang 421001, Peoples R China.

[Tan, Xiangshi] Fudan Univ, Dept Chem & Inst Biomed Sci, Shanghai 200433, Peoples R China.

通讯机构：

[Dr. Pengbing Mi; Dr. Pengbing Mi Dr. Pengbing Mi Dr. Pengbing Mi] D

[Prof. Dr. Ying-Wu Lin; Prof. Dr. Ying-Wu Lin Prof. Dr. Ying-Wu Lin Prof. Dr. Ying-Wu Lin] H

Hengyang Medical College School of Chemistry and Chemical Engineering, University of South China, Hengyang, 421001 P. R. China<&wdkj&>Key Lab of Protein Structure and Function of Universities in Hunan Province, University of South China, Hengyang, 421001 P. R. China<&wdkj&>Department of Pharmacy Hengyang Medicinal School, University of South China, Hengyang, Hunan, 421001 P. R. China

语种：

英文

关键词：

enzymes;model complex;molybdenum;oxygen atom transfer;nitrate reduction;S, N-bidentate ligands

期刊：

EUROPEAN JOURNAL OF INORGANIC CHEMISTRY

ISSN：

1434-1948

年：

2023

卷：

期：

页码：

e202200727-

DOI：

10.1002/ejic.202200727

基金类别：

National Natural Science Foundation of China [32171270, 21977042, 21977017]

机构署名：

本校为第一机构

院系归属：

化学化工学院

药学与生物科学学院

摘要：

Two new Mo‐complexes with N, S‐bidentate ligands were synthesized, and show good catalytic activity in the reduction of nitrate to nitrite. The addition of Lewis acid Sc(III) significantly accelerated the cycle rate of the Mo‐catalyst. Abstract Two readily‐accessible molybdenum complexes with low sterically hindered S, N‐bidentate ligands were designed for the reduction of nitrate to nitrite. The Lewis acid Sc(III) acted as a significant co‐catalyst to enhance the catalytic efficiency by activating the N−O bond of nitrate. This study ind...

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Lewis Acid-Assisted Molybdenum(VI) Complexes with S, N-bidentate Ligands to Reduce Nitrate

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