Due to its low thermal conductivity on average (~0.039 W/(m·K)), supercritical expanded polystyrene (PS) foam could be used as an insulation material in buildings to save energy and minimize the maintenance costs. However, the specific solubilizing and fast diffusing behavior of CO2 in PS limited the formation of micropores and the further increase of macropores, which resulted in on limited decrease in thermal conductivity. In this study, one-dimensional carbon nanotubes, two-dimensional graphene, and three-dimensional activated carbon were l...