A Rational Design of Metal-Organic Framework Nanozyme with High-Performance Copper Active Centers for Alleviating Chemical Corneal Burns

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成果类型：

期刊论文

作者：

Tang, Yonghua;Han, Yi;Zhao, Jiachen;Lv, Yufei;Fan, Chaoyu;...

通讯作者：

Lin, YH;Liu, Zuguo;Li, C

作者机构：

[Zhao, Jiachen; Fan, Chaoyu; Tang, Yonghua; Lin, YH; Zhang, Zhisen; Lin, Youhui] Xiamen Univ, Res Inst Biomimet & Soft Matter, Dept Phys, Fujian Prov Key Lab Soft Funct Mat Res, Xiamen 361005, Peoples R China.

[Li, Cheng; Han, Yi; Liu, Zuguo; Zheng, Lan] Xiamen Univ, Eye Inst, Sch Med, Fujian Prov Key Lab Ophthalmol & Visual Sci & Ocul, Xiamen 361102, Peoples R China.

[Li, Cheng; Han, Yi; Liu, Zuguo; Zheng, Lan] Xiamen Univ, Affiliated Xiamen Eye Ctr, Sch Med, Xiamen 361102, Peoples R China.

[Lin, YH; Lin, Youhui] Xiamen Univ, Natl Inst Data Sci Hlth & Med, Xiamen 361102, Peoples R China.

[Li, Cheng; Liu, Zuguo; Lv, Yufei] Univ South China, Affiliated Hosp 1, Dept Ophthalmol, Postdoctoral Mobile Stn Basic Med Sci,Hengyang Med, Hengyang 421001, Hunan, Peoples R China.

通讯机构：

[Liu, ZG; Li, C ; Lin, YH ] X

Xiamen Univ, Res Inst Biomimet & Soft Matter, Dept Phys, Fujian Prov Key Lab Soft Funct Mat Res, Xiamen 361005, Peoples R China.

Xiamen Univ, Eye Inst, Sch Med, Fujian Prov Key Lab Ophthalmol & Visual Sci & Ocul, Xiamen 361102, Peoples R China.

Xiamen Univ, Affiliated Xiamen Eye Ctr, Sch Med, Xiamen 361102, Peoples R China.

Xiamen Univ, Natl Inst Data Sci Hlth & Med, Xiamen 361102, Peoples R China.

语种：

英文

关键词：

Chemical ocular burn;Corneal diseases;Halogen;Metal–organic frameworks nanozyme;Superoxide dismutase

期刊：

纳微快报：英文版

ISSN：

2311-6706

年：

2023

卷：

期：

页码：

49-71

DOI：

10.1007/s40820-023-01059-9

基金类别：

National Key R&D Program of China [2020YFA0908100]; National Nature Science Foundation [12274356, 82070931, 82271045]; Fundamental Research Funds for the Central Universities [20720220022]; 111 Project [B16029]

机构署名：

本校为通讯机构

摘要：

Metal-organic frameworks (MOFs) have attracted significant research interest in biomimetic catalysis. However, the modulation of the activity of MOFs by precisely tuning the coordination of metal nodes is still a significant challenge. Inspired by metalloenzymes with well-defined coordination structures, a series of MOFs containing halogen-coordinated copper nodes (Cu-X MOFs, X = Cl, Br, I) are employed to elucidate their structure-activity relationship. Intriguingly, experimental and theoretical results strongly support that precisely tuning...

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A Rational Design of Metal-Organic Framework Nanozyme with High-Performance Copper Active Centers for Alleviating Chemical Corneal Burns

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