Synergistic Enhancement of Nitrogen Vacancies and Inverse Opal Structure in g-C3N4 for Efficient Photocatalytic Uranium Extraction

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成果类型：

期刊论文

作者：

Lijie Chen;Weilin Zhang;Xinyu Zhao;Guanghui Zhao;Le Li*;...

通讯作者：

Le Li

作者机构：

[Lijie Chen; Xinyu Zhao; Guanghui Zhao; Zhongran Dai] Key Discipline Laboratory for National Defense for Biotechnology in Uranium Mining and Hydrometallurgy, University of South China, Hengyang 421001, China

[Weilin Zhang] College of Public Health, Hengyang Medical School, University of South China, Hengyang 421001, Hunan, China

[Le Li] Key Discipline Laboratory for National Defense for Biotechnology in Uranium Mining and Hydrometallurgy, University of South China, Hengyang 421001, China<&wdkj&>College of Public Health, Hengyang Medical School, University of South China, Hengyang 421001, Hunan, China

通讯机构：

[Le Li] K

Key Discipline Laboratory for National Defense for Biotechnology in Uranium Mining and Hydrometallurgy, University of South China, Hengyang 421001, China<&wdkj&>College of Public Health, Hengyang Medical School, University of South China, Hengyang 421001, Hunan, China

语种：

英文

期刊：

Journal of Alloys and Compounds

ISSN：

0925-8388

年：

2025

页码：

183184

DOI：

10.1016/j.jallcom.2025.183184

基金类别：

CRediT authorship contribution statement Weilin Zhang: Investigation, Conceptualization. Xinyu Zhao: Visualization, Investigation. Lijie Chen: Writing – original draft, Validation, Investigation, Conceptualization. Zhongran Dai: Writing – review & editing, Supervision, acquisition. Guanghui Zhao: Visualization, Investigation. Le Li: Supervision, acquisition.

机构署名：

本校为第一且通讯机构

院系归属：

核资源工程学院

公共卫生学院

摘要：

Designing high-performance photocatalytic semiconductor catalysts remains a formidable challenge in energy conversion and environmental remediation. This study develops three-dimensionally ordered mesoporous carbon nitride photonic crystals (CNPC) with synergistic nitrogen vacancies and inverse opal structures via a hard-templating method using nitrogen-rich precursors. Urea-derived CNPCU achieves 96.95% U(Ⅵ) removal after 60 min photoactivation followed by 3 h dark reaction, substantially outperforming unmodified UCN. Mechanistic studies reve...

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Synergistic Enhancement of Nitrogen Vacancies and Inverse Opal Structure in g-C3N4 for Efficient Photocatalytic Uranium Extraction

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