Capturing critical gem-diol intermediates and hydride transfer for anodic hydrogen production from 5-hydroxymethylfurfural

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成果类型：

期刊论文

作者：

Fu, Guodong;Kang, Xiaomin;Zhang, Yan;Guo, Ying;Li, Zhiwei;...

通讯作者：

Liu, Jianwen;Fu, Xian-Zhu;Luo, JL

作者机构：

[Liu, Jianwen; Luo, Jing-Li; Guo, Ying; Fu, Guodong; Liu, JW; Wang, Lei; Luo, JL; Fu, Xian-Zhu] Shenzhen Univ, Coll Mat Sci & Engn, Guangdong Res Ctr Interfacial Engn Funct Mat, Shenzhen Key Lab Energy Electrocatalyt Mat, Shenzhen 518060, Peoples R China.

[Kang, Xiaomin] Univ South China, Sch Mech Engn, Hengyang 421001, Hunan, Peoples R China.

[Zhang, Yan] Shenzhen Bay Lab, Pingshan Translat Med Ctr, Shenzhen 518055, Guangdong, Peoples R China.

[Li, Zhiwei] Natl Supercomp Ctr Shenzhen, Shenzhen 518055, Peoples R China.

[Zhang, Jiujun] Fuzhou Univ, Coll Mat Sci & Engn, Fuzhou 350108, Peoples R China.

通讯机构：

[Liu, JW; Luo, JL ; Fu, XZ] S

Shenzhen Univ, Coll Mat Sci & Engn, Guangdong Res Ctr Interfacial Engn Funct Mat, Shenzhen Key Lab Energy Electrocatalyt Mat, Shenzhen 518060, Peoples R China.

语种：

英文

期刊：

Nature Communications

ISSN：

2041-1723

年：

2023

卷：

期：

页码：

8395

DOI：

10.1038/s41467-023-43704-2

基金类别：

Shenzhen Science and Technology Program (KQTD20190929173914967, ZDSYS20220527171401003) and the Senior Talent Research Start-up Fund of Shenzhen University (000263 and 000265) [22272108, 21975163, 22003041]; National Natural Science Foundation of China [KQTD20190929173914967, ZDSYS20220527171401003]; Shenzhen Science and Technology Program [000263, 000265J]; Senior Talent Research Start-up Fund of Shenzhen University; Instrumental Analysis Center of Shenzhen University

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本校为其他机构

院系归属：

机械工程学院

摘要：

The non-classical anodic H2 production from 5-hydroxymethylfurfural (HMF) is very appealing for energy-saving H2 production with value-added chemical conversion due to the low working potential (~0.1 V vs RHE). However, the reaction mechanism is still not clear due to the lack of direct evidence for the critical intermediates. Herein, the detailed mechanisms are explored in-depth using in situ Raman and Infrared spectroscopy, isotope tracking, and density functional theory calculations. The HMF is observed to form two unique inter-convertible ...

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Capturing critical gem-diol intermediates and hydride transfer for anodic hydrogen production from 5-hydroxymethylfurfural

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