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Electrochemical reactions of the Th4+/Th couple on the tungsten, aluminum and bismuth electrodes in chloride molten salt

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成果类型:
期刊论文
作者:
Liu, Kui;Yuan, Li-Yong;Liu, Ya-Lan;Zhao, Xiu-Liang;He, Hui;...
通讯作者:
Shi, Wei-Qun
作者机构:
[Liu, Ya-Lan; Yuan, Li-Yong; Liu, Kui; Chai, Zhi-Fang; Shi, Wei-Qun] Chinese Acad Sci, Inst High Energy Phys, Key Lab Nucl Radiat & Nucl Energy Technol, Beijing 100049, Peoples R China.
[Liu, Kui; Zhao, Xiu-Liang] Univ South China, Sch Nucl Sci & Technol, HengYang 421000, Peoples R China.
[Chai, Zhi-Fang] Soochow Univ, Sch Radiol & Interdisciplinary Sci, Suzhou 215123, Peoples R China.
[Liu, Ya-Lan; Ye, Guo-An; He, Hui] China Inst Atom Energy, Div Radiochem, Beijing 102413, Peoples R China.
通讯机构:
[Shi, Wei-Qun] C
Chinese Acad Sci, Inst High Energy Phys, Key Lab Nucl Radiat & Nucl Energy Technol, Beijing 100049, Peoples R China.
语种:
英文
期刊:
Electrochimica Acta
ISSN:
0013-4686
年:
2014
卷:
130
页码:
650-659
基金类别:
Major Research Plan "Breeding and Transmutation of Nuclear Fuel in Advanced Nuclear Fission Energy System" of the Natural Science Foundation of China [91226201, 91326202, 11105162, 11275219]; "Strategic Priority Research program" of the Chinese Academy of SciencesChinese Academy of Sciences [XDA030104]
机构署名:
本校为其他机构
院系归属:
核科学技术学院
摘要:
This work concerns the electrochemical behaviors of Th4+ on the tungsten, aluminum and bismuth electrodes in the LiCl-KCl eutectic, respectively, at 773 K. Cyclic voltammetry and square wave voltammetry were employed to investigate the cathodic reduction of Th4+. The results demonstrate that the reduction of Th4+ is a one step process with a transfer of 4 electrons. The reversibility of the Th4+/Th couple on the bismuth film and tungsten electrodes is directly confirmed by the CV. The diffusion coefficient is also calculated to be (2.23 ± 0.16...

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