The ecological hazards caused by the radioactive cesium (Cs) contaminants are long-standing and field-wide. In this study, the green rust (GR) was chemically formed and loaded onto the composite aluminosilicate materials (CAM) to enhance the adsorption capacities, environmental adaptability, and recyclability of CAM materials (GR-CAM) for Cs+ removal. The maximum monolayer adsorption capacities (mg/g) of GR-CAM for Cs+ adsorptions at pH of 2, 7, and 12 were 67.11, 104.93, and 129.03, respectively. The suitability of the pseudo-first-order kinetic model and Langmuir model for predicting Cs+ rem...