Sintering aids are commonly used to improve the sinterability of proton-conducting oxides, whereas the sintering aid elements are being used alone in previous research. In this study, a high-entropy design method for the BaCe0.4Zr0.4Y0.2O3 (BCZY) proton-conducting oxides sintering aid is proposed. In contrast to the use of sintering aids such as Ni, Fe, Cu, Co, and Zn alone, the high-entropy design allows for the simultaneous use of all five elements, resulting in the new composition BaCe0.4Zr0.4Y0.15Ni0.01Cu0.01Co0.01Fe0.01Zn0.01O3 (HE-BCZY). Compared to conventional BaCe0.4Zr0.4Y0.15M0.05O3 ...