Metal-Carboxyl Helical Chain Secondary Units Supported Ion-Exchangeable Anionic Uranyl–Organic Framework

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成果类型：

期刊论文

作者：

Mei, Lei;Liu, Kang;Wu, Si;Kong, Xiang-He;Hu, Kong-Qiu;...

通讯作者：

Shi, Wei-Qun

作者机构：

[Mei, Lei; Liu, Kang; Wu, Si; Kong, Xiang-He; Hu, Kong-Qiu; Yu, Ji-Pan; Chai, Zhi-Fang; Shi, Wei-Qun] Chinese Acad Sci, Inst High Energy Phys, Beijing 100049, Peoples R China

[Wu, Si; Nie, Chang-Ming] Univ South China, Sch Chem & Chem Engn, Hengyang 421001, Hunan, Peoples R China

[Chai, Zhi-Fang] Chinese Acad Sci, Engn Lab Adv Energy Mat, Ningbo Inst Ind Technol, Ningbo 315201, Zhejiang, Peoples R China

[Liu, Kang] Univ Chinese Acad Sci, Beijing 100039, Peoples R China

通讯机构：

[Shi, Wei-Qun] C

Chinese Acad Sci, Inst High Energy Phys, Beijing 100049, Peoples R China.

语种：

英文

关键词：

actinides;anionic framework;helical chain;ion exchange;uranyl–organic compounds

期刊：

CHEMISTRY-A EUROPEAN JOURNAL

ISSN：

0947-6539

年：

2019

卷：

期：

页码：

10309-10313

DOI：

10.1002/chem.201902180

基金类别：

We thank the support of this work by the Science Challenge Project (TZ2016004) and the National Natural Science Foundation of China (21671191, 21701178, and 11875057).

机构署名：

本校为其他机构

院系归属：

化学化工学院

摘要：

As a less explored avenue, actinide-based metal-organic frameworks (MOFs) are worth studying for the particularity of actinide nodes in coordination behaviour and assembly modes. In this work, an azobenzenetetracarboxylate-based anionic MOF supported by uranyl–carboxyl helical chain units was synthesized, incorporating linear uranyl as the metal centre. This kind of helical chain-type building unit is reported for the first time in uranyl-based MOFs. Structural analysis reveals that the formation of helical chain secondary units can be attribu...

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Metal-Carboxyl Helical Chain Secondary Units Supported Ion-Exchangeable Anionic Uranyl–Organic Framework

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