Defect engineering in metal-organic frameworks: a new strategy to develop applicable actinide sorbents

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成果类型：

期刊论文

作者：

Yuan, Liyong;Tian, Ming;Lan, Jianhui;Cao, Xingzhong;Wang, Xiaolin;...

通讯作者：

Shi, Weiqun

作者机构：

[Lan, Jianhui; Cao, Xingzhong; Yuan, Liyong; Chai, Zhifang; Shi, Weiqun; Tian, Ming] Chinese Acad Sci, Inst High Energy Phys, Lab Nucl Energy Chem, Beijing 100049, Peoples R China.

[Tian, Ming] Univ South China, Sch Chem & Chem Engn, Hengyang 421001, Hunan, Peoples R China.

[Wang, Xiaolin] China Acad Engn Phys, Inst Nucl Phys & Chem, Mianyang 621900, Sichuan, Peoples R China.

[Chai, Zhifang] Soochow Univ, Sch Radiol & Interdisciplinary Sci, Suzhou 215123, Peoples R China.

[Gibson, John K.] Lawrence Berkeley Natl Lab, Chem Sci Div, Berkeley, CA 94720 USA.

通讯机构：

[Shi, Weiqun] C

Chinese Acad Sci, Inst High Energy Phys, Lab Nucl Energy Chem, Beijing 100049, Peoples R China.

语种：

英文

期刊：

Chemical Communications

ISSN：

1359-7345

年：

2018

卷：

期：

页码：

370-373

DOI：

10.1039/c7cc07527h

基金类别：

National Natural Science Foundation of China [21471153, 21477130, U1432103, 21790373]; Youth Innovation Promotion Association, CAS; Science Challenge Project [JCKY2016212A504]; U.S. Department of Energy, Office of Science, Basic Energy Sciences [DE-SC0016568]

机构署名：

本校为其他机构

院系归属：

化学化工学院

摘要：

The preliminary results described here show that the adsorbability of uranyl ions by a highly stable MOF UiO-66 can be drastically enhanced by tailoring the missing-linker defects in this MOF. The combination of defect-induced functionality improvement with the acid-resistant nature of UiO-66 substantiates the applicability of this material...

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Defect engineering in metal-organic frameworks: a new strategy to develop applicable actinide sorbents

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