Dual Doping of N and F on Co3O4 to Activate the Lattice Oxygen for Efficient and Robust Oxygen Evolution Reaction

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成果类型：

期刊论文

作者：

Li, Chen;Ye, Beirong;Ouyang, Bo;Zhang, Tengfei;Tang, Tao;...

通讯作者：

Zhang, YQ;Xia, XH;Xia, Xinhui;Ouyang, B;Mei, BB

作者机构：

[Li, Chen; Zhang, Tengfei; Qiu, Zhong; Zhang, Yongqi; Ye, Beirong; Li, Sipu; Li, Yongqi; Tang, Tao] Univ Elect Sci & Technol China, Inst Fundamental & Frontier Sci, Chengdu 611731, Peoples R China.

[Li, Chen; Xia, Xinhui; Xia, XH] Zhejiang Univ Technol, Coll Mat Sci & Engn, Hangzhou 310014, Peoples R China.

[Li, Chen; Zhang, Yongqi; Xia, Xinhui; Xia, XH] Univ Elect Sci & Technol China, Yangtze Delta Reg Inst Huzhou, Huzhou 313002, Peoples R China.

[Ouyang, B; Ouyang, Bo] Nanjing Univ Sci & Technol, MIIT Key Lab Semicond Microstruct & Quantum Sensin, Nanjing 210094, Peoples R China.

[Chen, Renhong] Univ South China, Sch Elect Engn, Hengyang 421001, Peoples R China.

通讯机构：

[Mei, BB ] C

[Zhang, YQ ; Xia, XH] U

[Ouyang, B ] N

[Xia, XH ] Z

Univ Elect Sci & Technol China, Inst Fundamental & Frontier Sci, Chengdu 611731, Peoples R China.

语种：

英文

关键词：

co-doping;lattice oxygen mechanism;oxygen evolution reaction;spinel oxide;water splitting

期刊：

Advanced Materials

ISSN：

0935-9648

年：

2025

页码：

e2501381

DOI：

10.1002/adma.202501381

基金类别：

Zhejiang Provincial Natural Science Foundation of China [LD25B060003, LD25E020003]; National Natural Science Foundation of China [22379020, 52372235, 12304020]; Key Scientific Research Project of Hangzhou [2024SZD1B12]; Science and Technology Department of Zhejiang Province [2023C01231]; Science and Technology Project of Huzhou [2024GZ02]; State Key Laboratory of New Textile Materials and Advanced Processing Technologies [FZ2024009]; Hainan Province Science and Technology Special Fund [ZDYF2023GXJS148]; Natural Science Foundation of Jiangsu Province [BK20230909]; Fundamental Research Funds for the Central Universities [30923011013]

机构署名：

本校为其他机构

院系归属：

电气工程学院

摘要：

The oxygen evolution reaction (OER) is a pivotal process in numerous renewable energy conversion technologies. However, its sluggish intrinsic kinetics and intricate transfer process impede the efficient conversion of energy. Activating the lattice oxygen mechanism (LOM) is of paramount importance to break through the theoretical scaling relationship and boost the oxygen evolution catalytic activity. In this contribution, N and F are successfully introduced into Co(3)O(4) simultaneously as heteroatoms via a controllable plasma strategy to modulate the covalency property of metal-oxygen. Theore...

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Dual Doping of N and F on Co3O4 to Activate the Lattice Oxygen for Efficient and Robust Oxygen Evolution Reaction

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