Creating Lithium-Ion Electrolytes with Biomimetic Ionic Channels in Metal–Organic Frameworks

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成果类型：

期刊论文

作者：

Shen, Li;Wu, Hao Bin;Liu, Fang;Brosmer, Jonathan L.;Shen, Gurong;...

通讯作者：

Lu, Yunfeng;Wang, Ge;Dunn, Bruce

作者机构：

[Lu, Yunfeng; Shen, Li; Wang, Xiaofeng; Liu, Fang; Wu, Hao Bin] Univ Calif Los Angeles, Dept Chem & Biomol Engn, Los Angeles, CA 90095 USA.

[Wu, Hao Bin] Zhejiang Univ, Sch Mat Sci & Engn, Hangzhou 310027, Peoples R China.

[Zink, Jeffrey I.; Brosmer, Jonathan L.] Univ Calif Los Angeles, Dept Chem & Biochem, Los Angeles, CA 90095 USA.

[Wang, Xiaofeng] Univ South China, Sch Chem & Chem Engn, Hengyang 421001, Peoples R China.

[Cai, Mei; Xiao, Qiangfeng] Gen Motors Res & Dev Ctr, 30500 Mound Rd, Warren, MI 48090 USA.

通讯机构：

[Lu, Yunfeng; Wang, Ge; Dunn, Bruce] U

Univ Calif Los Angeles, Dept Chem & Biomol Engn, Los Angeles, CA 90095 USA.

Univ Sci & Technol Beijing, Sch Mat Sci & Engn, Beijing 100083, Peoples R China.

Univ Calif Los Angeles, Dept Mat Sci & Engn, Los Angeles, CA 90095 USA.

语种：

英文

关键词：

biomimetic ionic channels;lithium-ion electrolyte;lithium-metal batteries;metal–organic frameworks;open metal sites

期刊：

Advanced Materials

ISSN：

0935-9648

年：

2018

卷：

期：

页码：

e1707476

DOI：

10.1002/adma.201707476

基金类别：

L.S. and H.B.W. contributed equally to this work. This work was sponsored by the UCLA-HK Center for Graphene Technology and Energy Storage. J.B. and J.I.Z. gratefully acknowledge the support from the National Science Foundation under Grant No. 1362999.

机构署名：

本校为其他机构

院系归属：

化学化工学院

摘要：

Solid-state electrolytes are the key to the development of lithium-based batteries with dramatically improved energy density and safety. Inspired by ionic channels in biological systems, a novel class of pseudo solid-state electrolytes with biomimetic ionic channels is reported herein. This is achieved by complexing the anions of an electrolyte to the open metal sites of metal–organic frameworks (MOFs), which transforms the MOF scaffolds into ionic-channel analogs with lithium-ion conduction and low activation energy. This work suggests the em...

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Creating Lithium-Ion Electrolytes with Biomimetic Ionic Channels in Metal–Organic Frameworks

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