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The Delay Time Dependence of the Photoelectron Spectra and State Populations of Three-Level Ladder K-2 Molecule(1)

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成果类型:
期刊论文
作者:
Guo, Wei;Lu, Xingqiang*;Wang, Xinlin
通讯作者:
Lu, Xingqiang
作者机构:
[Guo, Wei; Wang, Xinlin] Univ South China, Sch Elect Engn, Hengyang 421001, Peoples R China.
[Guo, Wei] Dalian Inst Chem Phys, State Key Lab Mol React Dynam, Dalian 116023, Peoples R China.
[Lu, Xingqiang] Univ South China, Sch Nucl Sci & Technol, Hengyang 421001, Peoples R China.
通讯机构:
[Lu, Xingqiang] U
Univ South China, Sch Nucl Sci & Technol, Hengyang 421001, Peoples R China.
语种:
英文
关键词:
photoelectron spectra;state populations;time-dependent wave packet approach;three-level ladder K2 molecule
期刊:
Russian Journal of Physical Chemistry A
ISSN:
0036-0244
年:
2017
卷:
91
期:
2
页码:
366-372
基金类别:
National Science Foundation of ChinaNational Natural Science Foundation of China (NSFC) [11447020, 11174119]; Natural Science Foundation of Hunan provinceNatural Science Foundation of Hunan Province [2015JJ3104]
机构署名:
本校为第一且通讯机构
院系归属:
电气工程学院
核科学技术学院
摘要:
The delay time dependence of photoelectron spectra and state populations of three-level ladder K2 molecule is investigated by pump-probe pulses via time-dependent wave packet approach. The periodical motion of the wave packet with oscillating period 500 fs results in the periodical variation of photoelectron spectra. The photoelectron spectra show Autler-Townes double splitting at zero delay time, and no splitting at positive delay time. The periodical change of state populations with delay time can be ascribed to the coupling effect between the two pulses. It is found that the selectivity of ...

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