Amorphous Fe-Containing Phosphotungstates Featuring Efficient Peroxidase-like Activity at Neutral pH: Toward Portable Swabs for Pesticide Detection with Tandem Catalytic Amplification

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成果类型：

期刊论文

作者：

Zhu, Hengjia;Liu, Bangxiang;Wang, Mengzhu;Pan, Jianming;Xu, Lizhang;...

通讯作者：

Pan, Jianming(pjm@ujs.edu.cn);Xu, Lizhang(justxlz@ujs.edu.cn);Niu, Xiangheng(niuxiangheng@ujs.edu.cn)

作者机构：

[Xu, Lizhang; Niu, Xiangheng; Zhu, Hengjia] Jiangsu Univ, Sch Agr Engn, Zhenjiang 212013, Peoples R China.

[Pan, Jianming; Liu, Bangxiang; Hu, Panwang; Wang, Mengzhu; Niu, Xiangheng; Zhu, Hengjia] Jiangsu Univ, Inst Green Chem & Chem Technol, Sch Chem & Chem Engn, Zhenjiang 212013, Peoples R China.

[Niu, Xiangheng] Univ South China, Sch Publ Hlth, Hengyang Med Sch, Hengyang 421001, Peoples R China.

通讯机构：

[Jianming Pan] I

[Lizhang Xu; Xiangheng Niu] S

School of Agricultural Engineering, Jiangsu University, Zhenjiang 212013, China<&wdkj&>School of Agricultural Engineering, Jiangsu University, Zhenjiang 212013, China<&wdkj&>Institute of Green Chemistry and Chemical Technology, School of Chemistry and Chemical Engineering, Jiangsu University, Zhenjiang 212013, China<&wdkj&>School of Public Health, Hengyang Medical School, University of South China, Hengyang 421001, China<&wdkj&>Institute of Green Chemistry and Chemical Technology, School of Chemistry and Chemical Engineering, Jiangsu University, Zhenjiang 212013, China

语种：

英文

期刊：

Analytical Chemistry

ISSN：

0003-2700

年：

2023

卷：

期：

页码：

4776-4785

DOI：

10.1021/acs.analchem.3c00008

基金类别：

The work was supported by the Faculty of Agricultural Equipment of Jiangsu University (NZXB20210207), the Start-Up Research Fund of University of South China (221RGC011), the Fujian Key Laboratory of Functional Marine Sensing Materials, Minjiang University (MJUKF-FMSM2022010), the Postgraduate Research and Practice Innovation Program of Jiangsu Province (KYCX21_3381), and the National Natural Science Foundation of China (21605061).

机构署名：

本校为其他机构

院系归属：

公共卫生学院

摘要：

Peroxidase-mimetic materials are intensively applied to establish multienzyme systems because of their attractive merits. However, almost all of the nanozymes explored exhibit catalytic capacity only under acidic conditions. The pH mismatch between peroxidase mimics in acidic environments and bioenzymes under neutral conditions significantly restricts the development of enzyme-nanozyme catalytic systems especially for biochemical sensing. To solve this problem, here amorphous Fe-containing phosphotungstates (Fe-PTs) featuring high peroxidase ac...

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Amorphous Fe-Containing Phosphotungstates Featuring Efficient Peroxidase-like Activity at Neutral pH: Toward Portable Swabs for Pesticide Detection with Tandem Catalytic Amplification

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