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Cotransport of uranyl carbonate loaded on amorphous colloidal silica and strip-shaped humic acid in saturated porous media: Behavior and mechanism

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成果类型:
期刊论文
作者:
Hou, Wei;Lei, Zhiwu;Hu, Eming;Wang, Hongqiang;Wang, Qingliang;...
通讯作者:
Wang, Qingliang(670566869@qq.com)
作者机构:
[Hou, Wei; Wang, Hongqiang; Wang, Qingliang; Li, Hui; Zhang, Rui; Hu, Eming; Lei, Zhiwu] Univ South China, Sch Resource & Environm & Safety Engn, Hengyang 421001, Peoples R China.
[Hou, Wei; Wang, Qingliang] Univ South China, Cooperat Innovat Ctr Nucl Fuel Cycle Technol & Eq, Hengyang 421001, Peoples R China.
[Wang, Hongqiang] Univ South China, Hengyang Key Lab Soil Pollut Control & Remediat, Hengyang 421001, Peoples R China.
[Wang, Qingliang; Hu, Eming; Lei, Zhiwu] Univ South China, Hunan Key Lab Rare Met Minerals Exploitat & Geol, Hengyang 421001, Peoples R China.
通讯机构:
[Qingliang Wang] S
School of Resource & Environment and Safety Engineering, University of South China, Hengyang, 421001, China<&wdkj&>Cooperative Innovation Center for Nuclear Fuel Cycle Technology and Equipment, University of South China, Hengyang, 421001, China<&wdkj&>Hunan Key Laboratory of Rare Metal Minerals Exploitation and Geological Disposal of Wastes, University of South China, Hengyang, 421001, China
语种:
英文
关键词:
Amorphous silica;Cotransport;Humic acid;Radioactive pollution;Uranyl carbonate
期刊:
Environmental Pollution
ISSN:
0269-7491
年:
2021
卷:
285
页码:
117230
基金类别:
This work was financially supported by the National Natural Science Foundation of China ( 11675072 ), and the Hunan Provincial Innovation Foundation For Postgraduate ( CX20190719 ).
机构署名:
本校为第一机构
院系归属:
机械工程学院
摘要:
Uranyl carbonate (UC(VI)) is a stable form of uranyl (U(VI)) that widely coexists with amorphous colloidal silica (ACSi) and humic acid (HA) in carbonate-rich U-contaminated areas. In this context, the cotransport behavior and mechanism of UC(VI) with ACSi (100 mg L−1) and HA colloids in saturated porous media were systematically investigated. It was found that the ACSi and strip-shaped HA have a strong adsorption capacity for UC(VI), and their adsorption distribution coefficient (Kd) is 4–5 orders of magnitude higher than that of quartz sand...

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