Functional conversion of nickel-containing metalloproteins via molecular design: from a truncated acetyl-coenzyme A synthase to a nickel superoxide dismutase

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成果类型：

期刊论文

作者：

Liu, Yi;Wang, Qingli;Wei, Yaozhu;Lin, Ying-Wu;Li, Wei;...

通讯作者：

Tan, Xiangshi

作者机构：

[Wei, Yaozhu; Liu, Yi; Li, Wei; Tan, Xiangshi; Huang, Zhong-Xian] Fudan Univ, Dept Chem, Shanghai 200433, Peoples R China.

[Wei, Yaozhu; Liu, Yi; Li, Wei; Tan, Xiangshi; Huang, Zhong-Xian] Fudan Univ, Inst Biomed Sci, Shanghai 200433, Peoples R China.

[Wang, Qingli] Shandong Normal Univ, Coll Chem Chem Engn & Mat Sci, Jinan 250014, Peoples R China.

[Lin, Ying-Wu] Univ S China, Sch Chem & Chem Engn, Hengyang 421001, Peoples R China.

[Su, Ji-Hu] Univ Sci & Technol China, Dept Modern Phys, Hefei 230026, Peoples R China.

通讯机构：

[Tan, Xiangshi] F

Fudan Univ, Dept Chem, Shanghai 200433, Peoples R China.

语种：

英文

期刊：

Chemical Communications

ISSN：

1359-7345

年：

2013

卷：

期：

页码：

1452-1454

DOI：

10.1039/c2cc38224e

基金类别：

National Natural Science Foundation of ChinaNational Natural Science Foundation of China (NSFC) [91013001, 20771029, 31270869, 31070211]; Shanghai Leading Academic Discipline ProjectShanghai Leading Academic Discipline Project [B108]; Education Ministry of ChinaMinistry of Education, China [20100071110011]; high magnetic field laboratory of Chinese Academy of Science; Shanghai Synchrotron Radiation Facility (SSRF)

机构署名：

本校为其他机构

院系归属：

化学化工学院

摘要：

Truncated acetyl-coenzyme A synthase (ACS) was successfully converted into functional nickel superoxide dismutase (Ni-SOD) by molecular design and the designed metalloproteins possess new spectroscopic, structural, and electrochemical characteristics required for catalyzing O2 - disproportionation, and exhibit impressive Ni-SOD activity....

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Functional conversion of nickel-containing metalloproteins via molecular design: from a truncated acetyl-coenzyme A synthase to a nickel superoxide dismutase

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