Facile Synthesis of Hyperbranched Copolymers via an [A2+ B3] Click Polymerization Synthesized Reducible Hyperbranched Template

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成果类型：

期刊论文

作者：

Liu, Yuping;Ma, Wei;Dong, Zhen;Qiu, Nanting;Ma, Liwei;...

通讯作者：

Chen, Zhong-Ren(chenzr@sustech.edu.cn);Wei, Hua(weih@usc.edu.cn);Ma, Liwei(malw@lzu.edu.cn)

作者机构：

[Liu, Yuping; Dong, Zhen; Qiu, Nanting; Chen, Zhong-Ren] Shenzhen Grubbs Institute and Department of Chemistry, Southern University of Science and Technology, Shenzhen

518005, China

[Ma, Wei; Wei, Hua] Hunan Province Cooperative Innovation Center for Molecular Target New Drug Study, Department of Pharmacy and Pharmacology, University of South China, Hengyang

421001, China

[Ma, Liwei] College of Chemistry and Chemical Engineering, Lanzhou University, Gansu, Lanzhou

通讯机构：

[Liwei Ma] C

[Zhong-Ren Chen] S

[Hua Wei] H

Shenzhen Grubbs Institute and Department of Chemistry, Southern University of Science and Technology, Shenzhen 518005, China<&wdkj&>College of Chemistry and Chemical Engineering, Lanzhou University, Lanzhou, Gansu 730000, China<&wdkj&>Hunan Province Cooperative Innovation Center for Molecular Target New Drug Study & Department of Pharmacy and Pharmacology, University of South China, Hengyang, 421001, China<&wdkj&>College of Chemistry and Chemical Engineering, Lanzhou University, Lanzhou, Gansu 730000, China

语种：

英文

关键词：

acidic pH sensitivity;click polymerization;controlled drug release;degree of branch;hyperbranched polymer;reduction sensitivity

期刊：

ACS APPLIED POLYMER MATERIALS

ISSN：

2637-6105

年：

2021

卷：

期：

页码：

6375-6382

DOI：

10.1021/acsapm.1c01153

基金类别：

The authors acknowledge financial support from the National Natural Science Foundation of China (22075124, 51473072, and 21504035), the Shenzhen Special Fund (JCYJ20190809115013348), the Thousand Young Talent Program, and the Open Research Fund of State Key Laboratory of Polymer Physics and Chemistry, Changchun Institute of Applied Chemistry, Chinese Academy of Sciences.

机构署名：

本校为通讯机构

院系归属：

药学与生物科学学院

摘要：

Synthesis of multifunctional hyperbranched polymers (HPs) with simultaneously precisely modulated degrees of branch (DBs) and multibiorelevant signal-triggered sensitivities generally suffers from multistep preparation and purification procedures and uncontrolled DB. To develop a facile yet robust approach toward multifunctional HPs with a precisely modulated DB, we reported herein the synthesis of a reducible hyperbranched polymer template (HPT) with a fixed DB via an [A 2 + B 3 ]-based click polymerization and its further mediation of reversi...

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Facile Synthesis of Hyperbranched Copolymers via an [A2+ B3] Click Polymerization Synthesized Reducible Hyperbranched Template

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