Pressure-Induced Changes in Prussian Blue Analogues Na0.54Co1.23[Fe(CN)(6)]center dot 7.6H(2)O

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成果类型：

期刊论文

作者：

Xia, Yanfang;Mo, Jiajun;Zhang, Qinghang;Liu, Min;Peng, Anguo

通讯作者：

Min Liu

作者机构：

[Zhang, Qinghang; Peng, Anguo; Liu, Min; Mo, Jiajun; Xia, Yanfang] Univ South China, Coll Nucl Sci & Technol, Hengyang 421001, Peoples R China.

通讯机构：

[Min Liu] C

College of Nuclear Science and Technology, University of South China, Hengyang, China

语种：

英文

关键词：

Prussian blue analogues;pressure-induced;Mossbauer spectroscopy;magnetic properties

期刊：

Journal of Electronic Materials

ISSN：

0361-5235

年：

2022

卷：

期：

页码：

7150-7155

DOI：

10.1007/s11664-022-09953-5

基金类别：

National Natural Science Foundation of China [12105137, 11447231]; Natural Science Foundation of Hunan Province, China [2020JJ4517]; Research Foundation of Education Bureau of Hunan Province, China [19C1621, 19A434]; National Undergraduate Innovation and Entrepreneurship Training Program Support Projects of China [20200112, S202110555176]

机构署名：

本校为第一机构

院系归属：

核科学技术学院

摘要：

The effects of pressure on the microstructure and magnetic properties of Co-Fe bistable Prussian blue analogues (PBA) were investigated by Mossbauer spectroscopy and magnetic measurements. Na0.54Co1.23[Fe(CN)(6)]center dot 7.6H(2)O was prepared by the co-precipitation method and pressurized at 1-40 MPa using a supercritical CO2 extraction unit. All materials are face-centered cubic with a Neel temperature of about 14 K. The results showed that two electronic configurations existed in the NaCoFe-PBA system at room temperature: Fe-LS(III)-CN-Co-HS(II) and Fe-LS(II)-CN-Co-LS(III). The pressure in...

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Pressure-Induced Changes in Prussian Blue Analogues Na0.54Co1.23[Fe(CN)(6)]center dot 7.6H(2)O

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