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High performance self-assembled sulfidized nanoscale zero-valent iron for the immobilization of cadmium in contaminated sediments: Optimization, microbial response, and mechanisms

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成果类型:
期刊论文
作者:
Xu, Yiqun;Liu, Hongdou;Wen, Siqi;Guo, Jiaming;Shi, Xiaoyu;...
通讯作者:
Xue, WJ
作者机构:
[Lin, Weilong; Liu, Hongdou; Xue, Wenjing; Wen, Siqi; He, Qi; Shi, Xiaoyu; Xu, Yiqun; Guo, Jiaming] Yangzhou Univ, Coll Environm Sci & Engn, Yangzhou 225009, Peoples R China.
[Gao, Yang] Changsha Univ Sci & Technol, Sch Hydraul & Environm Engn, Changsha 410114, Peoples R China.
[Wang, Rongzhong] Univ South China, Sch Resource & Environm & Safety Engn, Hengyang 421001, Peoples R China.
通讯机构:
[Xue, WJ ] Y
Yangzhou Univ, Coll Environm Sci & Engn, Yangzhou 225009, Peoples R China.
语种:
英文
关键词:
Bacteria;Cadmium sulfide;Crystallinity;Efficiency;II-VI semiconductors;Iron;Nanotechnology;Physicochemical properties;Sediments;Bacterial community;Contaminated sediment;Immobilisation;Immobilization efficiency;Nano-scale zero valent irons;Nanoscale zero-valent iron;Overlying water;Performance;Precursor;Sulphidized nanoscale zero-valent iron;Cadmium;adsorbent;cadmium;calcium ion;citric acid;humic acid;iron;iron nanoparticle;magnesium ion;pentetic acid;potassium ion;sodium ion;sulfidized nanoscale zero valent iron;sulfur;unclassified drug;water;cadmium;iron;cadmium;complexation;immobilization;iron nanoparticle;microbial community;organic acid;performance assessment;sediment pollution;speciation (chemistry);adsorption;Article;bioremediation;cadmium poisoning;complex formation;controlled study;correlation analysis;correlation coefficient;crystal structure;energy dispersive X ray spectroscopy;environmental factor;environmental impact;environmental parameters;heavy metal removal;high resolution transmission electron microscopy;immobilization;incubation time;iron reducing bacterium;leaching;microbial activity;microbial community;microbial diversity;micromorphology;nonhuman;oxidation;particle size;pH;physical chemistry;precipitation;precursor;process optimization;prokaryotes by metabolism;scanning electron microscopy;sediment;Shannon index;sulfate reducing bacterium;toxic concentration;transmission electron microscopy;water contamination;water sediment ratio;X ray diffraction;X ray photoemission spectroscopy;chemistry;water pollutant;Adsorption;Cadmium;Iron;Water;Water Pollutants, Chemical
期刊:
Journal of Hazardous Materials
ISSN:
0304-3894
年:
2024
卷:
469
页码:
134022
基金类别:
This study was financially supported by the Program for the National Natural Science Foundation of China (42107415) and Natural Science Foundation of Jiangsu Province (BK20210830).
机构署名:
本校为其他机构
摘要:
Sulfidized nanoscale zero-valent iron (S-nZVI) showed excellent removal capacity for cadmium (Cd) in aqueous phase. However, the remediation effects of S-nZVI on Cd-contaminated sediment and its interactions with microorganisms in relation to Cd fate remain unclear. The complexity of the external environment posed a challenge for Cd remediation. This study synthesized S-nZVI with different S and Fe precursors to investigate the effect of precursors and applied the optimal material to immobilize Cd in sediments. Characterization analysis reveale...

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