Small-Molecule Hole Transport Materials for >26% Efficient Inverted Perovskite Solar Cells

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成果类型：

期刊论文

作者：

Zeng, Jie;Liu, Zhixin;Wang, Deng;Wu, Jiawen;Zhu, Peide;...

通讯作者：

Wang, Xingzhu;Zhang, Yong;Xu, BM;Jen, AKY;Yan, L;Wang, XZ

作者机构：

[Xu, Baomin; Wu, Jiawen; Hu, Bihua; Wang, Xingzhu; Liu, Zhixin; Zhang, Yong; Wang, Deng; Wang, XZ; Bao, Yuqi; Zhu, Peide; Zeng, Jie] Southern Univ Sci & Technol, Dept Mat Sci & Engn, Shenzhen 518055, Peoples R China.

[Xu, Baomin; Wu, Jiawen; Hu, Bihua; Wang, Xingzhu; Liu, Zhixin; Zhang, Yong; Wang, Deng; Wang, XZ; Bao, Yuqi; Zhu, Peide; Zeng, Jie] Southern Univ Sci & Technol, Shenzhen Engn Res & Dev Ctr Flexible Solar Cells, Shenzhen 518055, Peoples R China.

[Wang, Deng; Jen, Alex K. -Y.; Jen, AKY; Zeng, Jie] City Univ Hong Kong, Dept Mat Sci & Engn, Kowloon, Hong Kong 999077, Peoples R China.

[Yan, Lei; Guo, Xiaoyu; Yan, L] Xiangtan Univ, Sch Phys & Optoelect, Xiangtan 411105, Peoples R China.

[Qu, Geping] Southern Univ Sci & Technol, Dept Chem, Shenzhen 518055, Peoples R China.

通讯机构：

[Xu, BM ; Zhang, Y; Wang, XZ] S

[Wang, XZ ] U

[Jen, AKY ] C

[Yan, L ] X

Southern Univ Sci & Technol, Dept Mat Sci & Engn, Shenzhen 518055, Peoples R China.

语种：

英文

期刊：

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY

ISSN：

0002-7863

年：

2025

卷：

147

期：

页码：

725–733

DOI：

10.1021/jacs.4c13356

基金类别：

National Natural Science Foundation of China [2021YFB3800101]; National Key Research and Development Project funding from the Ministry of Science and Technology of China [62204108]; National Natural Science Foundation of China [JCYJ20220818100211025, SGDX20230116091649013, JCYJ20220530113205013]; Shenzhen Science and Technology Innovation Committee [2023B1515120031, 2021A1515110628, 2023A1515012797]; Guangdong Basic and Applied Basic Research Foundation [2023JJ50132]; Natural Science Foundation of Hunan Province, China [G03034K001]; SUSTech Energy Institute for Carbon Neutrality (High level of special funds); Center for Computational Science and Engineering at SUSTech

机构署名：

本校为通讯机构

院系归属：

电气工程学院

摘要：

Chemically modifiable small-molecule hole transport materials (HTMs) hold promise for achieving efficient and scalable perovskite solar cells (PSCs). Compared to emerging self-assembled monolayers, small-molecule HTMs are more reliable in terms of large-area deposition and long-term operational stability. However, current small-molecule HTMs in inverted PSCs lack efficient molecular designs that balance both the charge transport capability and interface compatibility, resulting in a long-standing stagnation of power conversion efficiency (PCE) ...

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Small-Molecule Hole Transport Materials for >26% Efficient Inverted Perovskite Solar Cells

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