Construction of a myoglobin scaffold-based biocatalyst for the biodegradation of sulfadiazine and sulfathiazole

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成果类型：

期刊论文

作者：

Zhang, Weikang;Lin, Yingwu;Meng, Xiangmin;Wang, Qiaoning;Chen, Lingxin;...

通讯作者：

Xu, JK;Chen, LX

作者机构：

[Zhang, Weikang; Xu, Jiakun] Chinese Acad Fishery Sci, Yellow Sea Fisheries Res Inst, State Key Lab Mariculture Biobreeding & Sustainabl, Lab Marine Drugs & Byprod Pilot Natl Lab Marine Sc, Qingdao 266071, Peoples R China.

[Zhang, Weikang; Meng, Xiangmin] Qingdao Univ Sci & Technol, Coll Marine Sci & Biol Engn, Qingdao 266042, Peoples R China.

[Lin, Yingwu] Univ South China, Sch Chem & Chem Engn, Hengyang 421001, Peoples R China.

[Chen, Lingxin; Chen, LX; Wang, Qiaoning] Chinese Acad Sci, Yantai Inst Coastal Zone Res, Res Ctr Coastal Environm Engn & Technol, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai 264003, Peoples R China.

通讯机构：

[Xu, JK ; Chen, LX ] C

Chinese Acad Fishery Sci, Yellow Sea Fisheries Res Inst, State Key Lab Mariculture Biobreeding & Sustainabl, Lab Marine Drugs & Byprod Pilot Natl Lab Marine Sc, Qingdao 266071, Peoples R China.

Chinese Acad Sci, Yantai Inst Coastal Zone Res, Res Ctr Coastal Environm Engn & Technol, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai 264003, Peoples R China.

语种：

英文

关键词：

Biocatalysis;Biodegradation;Directed evolution;Myoglobin;Sulfonamides

期刊：

Journal of Hazardous Materials

ISSN：

0304-3894

年：

2024

卷：

465

页码：

133147

DOI：

10.1016/j.jhazmat.2023.133147

基金类别：

National Key R & D Program of China [2022YFC2807500]; National Natural Science Foundation of China [32171270]; Central Public-Interest Scientific Institution Basal Research Fund, CAFS [2023TD71]

机构署名：

本校为其他机构

院系归属：

化学化工学院

摘要：

Sulfonamide antibiotics, a family of broad-spectrum antibiotic drugs, are increasingly used in aquaculture and are frequently detected in aquatic environments. This poses a potential threat to organisms and may cause the evolution of antimicrobial resistance. Therefore, it is important to develop an environmentally friendly and efficient biocatalyst to degrade sulfonamides (SAs) such as sulfadiazine (SD) and sulfathiazole (ST). Here, we realized the direct and efficient degradation of SD and ST using a hydrogen peroxide-dependent artificial cat...

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Construction of a myoglobin scaffold-based biocatalyst for the biodegradation of sulfadiazine and sulfathiazole

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