Highly ordered 2D honeycomb polyoxometalate clusterphene for efficient photocatalytic degradation of organic pollutants: Mechanism, pathways, and toxicity evaluation

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成果类型：

期刊论文

作者：

Zhang, Xinyi;Xu, Yiguo;Guo, Rongshuo;Chen, Yinxiang*;Zhang, Ye

通讯作者：

Zhang, Y;Chen, Yinxiang

作者机构：

[Guo, Rongshuo; Zhang, Xinyi; Zhang, Ye; Zhang, Y] Univ South China, Sch Chem & Chem Engn, Lab Optoelect Technol Low Dimens Nanomat, Hengyang 421001, Peoples R China.

[Chen, Yinxiang; Zhang, Ye; Zhang, Y] Univ South China, Sch Resources Environm & Safety Engn, Hengyang 421001, Peoples R China.

[Xu, Yiguo] Southern Univ Sci & Technol, Acad Adv Interdisciplinary Studies, Shenzhen 518055, Peoples R China.

通讯机构：

[Chen, YX; Zhang, Y ] U

Univ South China, Sch Chem & Chem Engn, Lab Optoelect Technol Low Dimens Nanomat, Hengyang 421001, Peoples R China.

Univ South China, Sch Resources Environm & Safety Engn, Hengyang 421001, Peoples R China.

语种：

英文

关键词：

Polyoxometalate clusterphene;Highly ordered structure;Photocatalytic degradation;DFT calculations;Organic pollutants

期刊：

Applied Surface Science

ISSN：

0169-4332

年：

2024

卷：

656

页码：

159675

DOI：

10.1016/j.apsusc.2024.159675

基金类别：

CRediT authorship contribution statement Xinyi Zhang: Writing – original draft, Investigation, Data curation. Yiguo Xu: Software, Formal analysis. Rongshuo Guo: Formal analysis, Data curation. Yinxiang Chen: Methodology, Conceptualization. Ye Zhang: Writing – review & editing, acquisition, Conceptualization, Supervision, Methodology.

机构署名：

本校为第一且通讯机构

院系归属：

化学化工学院

摘要：

Self -assembled nanomaterials have aroused enormous interest owing to their enhanced physicochemical properties as compared to monomers. Herein, two-dimensional Nd-based polyoxometalate clusterphene (Nd-POMCene) with a highly ordered honeycomb structure is synthesized by self -assembly, which is demonstrated with efficient photocatalytic degradation performance towards organic dyes, such as Rhodamine B (RhB), methylene blue, and crystal violet. Especially, RhB can be totally photodegraded by Nd-POMCene under the simulated sunlight within 1 h while a degraded efficiency of 97.50 % can be achiev...

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Highly ordered 2D honeycomb polyoxometalate clusterphene for efficient photocatalytic degradation of organic pollutants: Mechanism, pathways, and toxicity evaluation

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