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Experimental and computational study on the mechanism of iodine vapour adsorption by modified activated carbon fibers at different scales

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成果类型:
期刊论文
作者:
Yang, Xiaomin;Wu, Hui;Xie, Dong
通讯作者:
Xie, D
作者机构:
[Yang, Xiaomin] Univ South China, Sch Resource Environm & Safety Engn, Hengyang 421001, Peoples R China.
[Xie, D; Xie, Dong; Wu, Hui; Yang, Xiaomin] Natl & Local Joint Engn Res Ctr Airborne Pollutant, Hengyang 421001, Peoples R China.
[Xie, D; Xie, Dong; Wu, Hui] Univ South China, Sch Civil Engn, Hengyang 421001, Peoples R China.
通讯机构:
[Xie, D ] N
Natl & Local Joint Engn Res Ctr Airborne Pollutant, Hengyang 421001, Peoples R China.
Univ South China, Sch Civil Engn, Hengyang 421001, Peoples R China.
语种:
英文
关键词:
Iodine vapour;Modified activated carbon fibers;COMSOL simulation;GCMC simulation
期刊:
Journal of Radioanalytical and Nuclear Chemistry
ISSN:
0236-5731
年:
2023
卷:
332
期:
11
页码:
4427-4439
基金类别:
This work was supported by the National Natural Science Foundation of China (Grant Number 12275122 and U1867221). [12275122, U1867221]; National Natural Science Foundation of China
机构署名:
本校为第一且通讯机构
院系归属:
土木工程学院
摘要:
The effective capture of iodine vapour, a potential threat of environment and human health, is crucial for efficiently managing nuclear waste gases. Herein, the adsorption property of iodine vapour on modified activated carbon fibers was investigated using adsorption experiment and simulation methods, to explain the adsorption mechanism at different scales. Preliminary results hint that the ideal adsorbent should have lower density, higher adsorption coefficient and taller poriness, and more pores between 1.6 and 1.9 nm. Compared with KOH modification, microwave modification can effectively im...

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