High-efficiency ammonia synthesis via electrochemical nitrate reduction over Co3O4 nanoarrays by B doping - 成果

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High-efficiency ammonia synthesis via electrochemical nitrate reduction over Co₃O₄ nanoarrays by B doping

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成果类型：

期刊论文

作者：

Deng, Zhiqin;Liu, Heng;Wang, Huiyong;Ma, Chaoqun;Du, Juan*;...

通讯作者：

Du, Juan;Zheng, BZ;Ma, CQ

作者机构：

[Deng, Zhiqin; Liu, Heng] Univ South China, Sch Chem & Chem Engn, Hengyang 421001, Hunan, Peoples R China.

[Du, Juan; Deng, Zhiqin; Zheng, BZ; Zheng, Baozhan] Sichuan Univ, Coll Chem, Chengdu 610064, Sichuan, Peoples R China.

[Wang, Huiyong] Henan Normal Univ, Coll Chem & Chem Engn, Xinxiang 453007, Henan, Peoples R China.

[Ma, Chaoqun; Ma, CQ] Univ Sci & Technol Beijing, Sch Mat Sci & Engn, Beijing 100083, Peoples R China.

通讯机构：

[Du, J; Zheng, BZ ] S

[Ma, CQ ] U

Sichuan Univ, Coll Chem, Chengdu 610064, Sichuan, Peoples R China.

Univ Sci & Technol Beijing, Sch Mat Sci & Engn, Beijing 100083, Peoples R China.

语种：

英文

期刊：

无机化学前沿

ISSN：

2052-1553

年：

2024

卷：

期：

页码：

2339-2345

DOI：

10.1039/d4qi00310a

基金类别：

Henan Normal University [21876117]; National Natural Science Foundation of China [2021YB05]; Open Research Fund of School of Chemistry and Chemical Engineering, Henan Normal University

机构署名：

本校为第一机构

院系归属：

化学化工学院

摘要：

Electrochemical conversion of nitrate to valuable ammonia (NH3) is a green and widely used approach to NH3 synthesis that can be an attractive and complementary alternative to the Haber-Bosch process. However, due to the multi-step reactions in the nitrate reduction pathway, there are still challenges in developing efficient catalysts that can selectively guide the reaction route towards NH3. Herein, B doping is proposed as an effective strategy to enhance nitrate conversion to NH(3 )on the Co3O4 nanoarrays, which not only improves the electrical conductivity of Co3O4, but also lowers the ener...

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High-efficiency ammonia synthesis via electrochemical nitrate reduction over Co₃O₄ nanoarrays by B doping

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