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Modulating the electronic structure of a hydrogen-bonded organic framework to enhance uranium removal via the hydrogen evolution reaction

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成果类型:
期刊论文
作者:
Zhang, Qingsong*;Miao, Yuyang;Xiao, Yang;Hu, Jianwei;Gong, Haiyi;...
通讯作者:
Zhang, Qingsong;Zeng, QY;Xiao, Y
作者机构:
[Zeng, Qingyi; Miao, Yuyang; Zhang, Qingsong; Gong, Haiyi; Hu, Jianwei] Univ South China, Sch Resource & Environm & Safety Engn, Hengyang 421001, Peoples R China.
[Xiao, Y; Xiao, Yang] Univ South China, Sch Nucl Sci & Technol, Hengyang 421001, Peoples R China.
通讯机构:
[Zeng, QY ; Xiao, Y ; Zhang, QS] U
Univ South China, Sch Resource & Environm & Safety Engn, Hengyang 421001, Peoples R China.
Univ South China, Sch Nucl Sci & Technol, Hengyang 421001, Peoples R China.
语种:
英文
期刊:
无机化学前沿
ISSN:
2052-1545
年:
2025
卷:
12
期:
5
页码:
1935-1949
基金类别:
National Natural Science Foundation of China [12305387, 52170083]; National Natural Science Foundation of China [2022JJ40376]; Hunan Provincial Natural Science Foundation of China [21B0441]; Research Foundation of Education Bureau of Hunan Province, China [2022RC1125]; Science and Technology Innovation Program of Hunan Province
机构署名:
本校为第一且通讯机构
院系归属:
核科学技术学院
摘要:
Photocatalytic extraction of uranium from solution is one of the most promising technologies for uranium recovery. However, the presence of axial bonds between the two oxygen atoms in UO 2 2+ creates a high activation barrier for electron transfer, which hinders the reduction of UO 2 2+ , making it more challenging to reduce U( VI ) to U( IV ) with conventional photocatalysis. Herein, an ingenious strategy for the efficient removal of uranium from aqueous solutions, utilizing the photocatalytic hydrogen evolution reaction (HER) process, is prop...

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